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COATINGS

TECHNOLOGY

HANDBOOK

Third

Edition

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A CRC title, part of the Taylor & Francis imprint, a member of the Taylor & Francis Group, the academic division of T&F Informa plc.

COATINGS

TECHNOLOGY

HANDBOOK

Third

Edition

Edited by

Arthur A. Tracton

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Published in 2006 by CRC Press

Taylor & Francis Group

6000 Broken Sound Parkway NW, Suite 300 Boca Raton, FL 33487-2742

© 2006 by Taylor & Francis Group, LLC CRC Press is an imprint of Taylor & Francis Group No claim to original U.S. Government works

Printed in the United States of America on acid-free paper 10 9 8 7 6 5 4 3 2 1

International Standard Book Number-10: 1-57444-649-5 (Hardcover) International Standard Book Number-13: 978-1-57444-649-4 (Hardcover)

This book contains information obtained from authentic and highly regarded sources. Reprinted material is quoted with permission, and sources are indicated. A wide variety of references are listed. Reasonable efforts have been made to publish reliable data and information, but the author and the publisher cannot assume responsibility for the validity of all materials or for the consequences of their use.

No part of this book may be reprinted, reproduced, transmitted, or utilized in any form by any electronic, mechanical, or other means, now known or hereafter invented, including photocopying, microfilming, and recording, or in any information storage or retrieval system, without written permission from the publishers.

01923, 978-750-8400. CCC is a not-for-profit organization that provides licenses and registration for a variety of users. For organizations that have been granted a photocopy license by the CCC, a separate system of payment has been arranged.

Trademark Notice: Product or corporate names may be trademarks or registered trademarks, and are used only for

identification and explanation without intent to infringe.

Library of Congress Cataloging-in-Publication Data Catalog record is available from the Library of Congress

Visit the Taylor & Francis Web site at and the CRC Press Web site at

Taylor & Francis Group is the Academic Division of T&F Informa plc.

For permission to photocopy or use material electronically from this work, please access www.copyright.com

(http://www.copyright.com/) or contact the Copyright Clearance Center, Inc. (CCC) 222 Rosewood Drive, Danvers, MA

http://www.taylorandfrancis.com http://www.crcpress.com

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v

Preface to Third Edition

The world of coatings is very broad. The application techniques are many, and the uses are numerous. Technical people need to be aware of many things. One study said that a coating chemist must be proficient in 27 different disciplines. This book is directed at supplying a broad cross-index of some of the different aspects to help the technical person. It is not meant to be an in-depth treatise on any subject. It is meant to give insight into the various subjects covered. The chapter authors or the editor may be contacted for more information or direction on the subjects.

To aid the person involved in coatings, inks, or adhesives, be they chemists, engineers, technicians, researchers, or manufacturers, chapters are given in the areas of fundamentals and testing, coating and processing, techniques and materials, and surface coatings. Each section contains information to expand the awareness and knowledge of someone practicing in the field. The objective is to help people solve problems and increase their level of technology. With time, technology increases, as shown by the chapter on statistical design of experiments, and the chapter on using equipment to determine ultraviolet (UV) resistance. Newer materials such as fluorocarbon resins, polyurethane thickeners, and high-temperature pigments are included as well as older materials such as alkyds, clays, and driers.

To accomplish the presentation of technology, this book has been expanded to 118 chapters by adding new material and updating other material. Hopefully, the reader will expand his or her knowledge and further push the envelope of technology.

The editor gratefully acknowledges the many contributions of the chapter authors and the publishers who have made this book possible.

Arthur A. Tracton

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vii

Contributors

N. J. Abbott

Albany International Research Company

Dedham, Massachusetts

Harold Van Aken

GretagMacbeth

New Windsor, New York

Walter Alina

General Magnaplate Corporation Linden, New Jersey

Mark J. Anderson

Stat-Ease, Inc. Minneapolis, Minnesota

Robert D. Athey, Jr.

Athey Technologies El Cerrito, California

Brian E. Aufderheide

W. H. Brady Company Milwaukee, Wisconsin

Bruce R. Baxter

Specialty Products, Inc. Lakewood, Washington

William F. Beach

Bridgeport, New Jersey

Edward A. Bernheim

Exxene Corporation Corpus Christi, Texas

Deepak G. Bhat

GTE Valenite Corporation Troy, Michigan

Thomas P. Blomstrom

Monsanto Chemical Company Springfield, Massachusetts

Kenneth Bourlier

Union Carbide Corporation Bound Brook, New Jersey

J. David Bower

Hoechst Celanese Corporation Somerville, New Jersey

Donald L. Brebner

E. I. du Pont de Nemours & Company

Wilmington, Delaware

Patrick Brennan

Q-Panel Lab Products Cleveland, Ohio

George E. F. Brewer

George E. F. Brewer Coating Consultants Birmingham, Michigan

Lisa A. Burmeister

Aqualon Company Wilmington, Delaware

Peter A. Callais

Pennwalt Corporation Buffalo, New York

Naomi Luft Cameron

Datek Information Services Newtonville, Massachusetts

Robert W. Carpenter

Windsor Plastics, Inc. Evansville, Indiana

Chi-Ming Chan

Raychem Corporation Menlo Park, California

Gary W. Cleary

Cygnus Research Corporation Redwood City, California

Carl A. Dahlquist

3M Company St. Paul, Minnesota

B. Davis

ABM Chemicals Limited Stockport, Cheshire, England

Richey M. Davis

Hercules Incorporated Wilmington, Delaware

David R. Day

Micromet Instruments, Inc. Cambridge, Massachusetts

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viii

Marcel Dery

Chemical Fabrics Corporation Merrimack, New Hampshire

Arnold H. Deutchman

BeamAlloy Corporation Dublin, Ohio

John W Du

BYK-Chemie USA Wallingford, Connecticut

Richard P. Eckberg

General Electric Company Schenectady, New York

Jesse Edenbaum

Consultant

Cranston, Rhode Island

Eric T. Everett

Q-Panel Lab Products Cleveland, Ohio

Carol Fedor

Q-Panel Lab Products Cleveland, Ohio

William C. Feist

Consultant

Middleton, Wisconsin

R. H. Foster

Eval Company of America Lisle, Illinois

James D. Gasper

ICI Resins US

Wilmington, Massachusetts

Sam Gilbert

Sun Chemical Corporation Cincinnati, Ohio

K. B. Gilleo

Sheldahl, Inc. Northfield, Minnesota

William S. Gilman

Gilman & Associates South Plainfield, New Jersey

F. A. Goossens

Stork Brabant

Boxmeer, The Netherlands

Joseph Green

FMC Corporation Princeton, New Jersey

Douglas Grossman

Q-Panel Lab Products Cleveland, Ohio

Clive H. Hare

Coating System Design, Inc. Lakeville, Massachusetts

William F. Harrington,

Jr.

Uniroyal Adhesives and Sealants Company, Inc.

Mishawaka, Indiana

J. Rufford Harrison

E. I. du Pont de Nemours & Company

Wilmington, Delaware

Helen Hatcher

Johnson Matthey Pigments & Dispersions

Kidsgrove, Stoke-on-Trent, Staffs, United Kingdom

Jack Hickey

International Paint Company Union, New Jersey

Herman Hockmeyer

Hockmeyer Equipment Corporation

Elizabeth City, North Carolina

Krister Holmberg

Chalmers University of Technology Göteborg, Sweden

Albert G. Hoyle

Hoyle Associates Lowell, Massachusetts

H. F. Huber

Hüls Troisdorf AG Troisdorf/Marl, Germany

Michael Iskowitz

Kop-Coat Marine Group Rockaway, New Jersey

Joseph L. Johnson

Aqualon Company Wilmington, Delaware

Stephen L. Kaplan

Plasma Science, Inc. Belmont, California

Douglas S. Kendall

National Enforcement Investigations Center U.S. Environmental Protection

Agency

Denver Federal Center Denver, Colorado

Ashok Khokhani

Engelhard Corporation Iselin, New Jersey

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ix

Carol D. Klein

Spectra Colors Corporation Kearny, New Jersey

Lisa C. Klein

Ceramic and Materials Engineering

Rutgers — The State University of New Jersey

Piscataway, New Jersey

Joseph V. Koleske

Charleston, West Virginia

Alan Lambuth

Boise Cascade Boise, Idaho

Kenneth Lawson

DeSoto, Inc. Des Plaines, Illinois

B. H. Lee

Ciba-Geigy Corporation Ardsley, New York

Peter A. Lewis

Sun Chemical Corporation Cincinnati, Ohio

Raimond Liepins

Los Alamos National Laboratory Los Alamos, New Mexico

H. Thomas Lindland

Flynn Burner Corporation New Rochelle, New York

Harry G. Lippert

Extrusion Dies, Inc. Chippewa Falls, Wisconsin

Ronald A. Lombardi

ICI Resins US Wilmington, Massachusetts

Donald M. MacLeod

Industry Tech Oldsmar, Florida

Algirdas Matukonis

Kaunas Technical University Kaunas, Lithuania

John A. McClenathan

IMD Corporation Birmingham, Alabama

Christopher W.

McGlinchey

The Metropolitan Museum of Art

New York, New York

Frederic S. McIntyre

Acumeter Laboratories, Inc. Marlborough, Massachusetts

Timothy B. McSweeney

Screen Printing Association International Fairfax, Virginia

R. Milker

Lohmann GmbH Neuwied, Germany

Samuel P. Morell

S. P. Morell and Company Armonk, New York

Wayne E. Mozer

Oxford Analytical, Inc. Andover, Massachusetts

Helmut W. J. Müller

BASF AG

Ludwigshafen/Rhein, Germany

Richard Neumann

Windmöller & Hölscher Lengerich/Westfalen, Germany

Robert E. Norland

Norland Products, Inc. North Brunswick, New Jersey

Milton Nowak

Troy Chemical Newark, New Jersey

Michael O’Mary

The Armoloy Corporation DeKalb, Illinois

Robert J. Partyka

BeamAlloy Corporation Dublin, Ohio

John A. Pasquale III

Liberty Machine Company Paterson, New Jersey

Patrick Patton

Q-Panel Lab Products Cleveland, Ohio

Detlef van Peij

Solventborne Coatings — Europe Elementis GmbH Cologne, Germany

Kim S. Percell

Witco Corporation Memphis, Tennessee

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x

Edwin P. Plueddemann

Dow Corning Corporation Midland, Michigan

Liudas Pranevicius

Vytautas Magnus University Kaunas, Lithuania

Charles P. Rader

Advanced Elastomer Systems, L.P.

Akron, Ohio

Valentinas Rajeckas

Kaunas Polytechnic University Kaunas, Lithuania

H. Randhawa

Vac-Tec Systems, Inc. Boulder, Colorado

Richard Rathmell

Londonderry, New Hampshire

Donald A. Reinke

Oliver Products Company (Retired)

Grand Rapids, Michigan

Peter W. Rose

Plasma Science, Inc. Belmont, California

D. Satas

Satas & Associates Warwick, Rhode Island

Milton C. Schmit

Plymouth Printing Company, Inc.

Cranford, New Jersey

Jaykumar (Jay) J. Shah

Decora

Fort Edward, New York

Douglas N. Smith

Waterborne Coatings — Global Elementis GmbH

Cologne, Germany

Steve Stalker

ITW Industrial Finishing Glendale Heights, Illinois

Henry R. Stoner

Henry R. Stoner Associates North Plainfield, New Jersey

D. Stoye

Hüls Troisdorf AG Troisdorf/Marl, Germany

Larry S. Timm

Findley Adhesives, Inc. Wauwatosa, Wisconsin

Harry H. Tomlinson

Witco Corporation Memphis, Tennessee

Arthur A. Tracton

Consultant

Bridgewater, New Jersey

George D. Vaughn

Surface Specialties Melamines Springfield, Massachusetts

A. Vaˇskelis

Lithuanian Academy of Sciences Vilnius, Lithuania

Subbu Venkatraman

Raychem Corporation Menlo Park, California

Theodore G.

Vernardakis

BCM Inks USA, Inc. Cincinnati, Ohio

Lawrence R. Waelde

Troy Corporation Florham Park, New Jersey

Leonard E. Walp

Witco Corporation Memphis, Tennessee

Patrick J. Whitcomb

Stat-Ease, Inc. Minneapolis, Minnesota

K. Winkowski

ISP Corporation Piscataway, New Jersey

Kurt A. Wood

Arkema, Inc.

King of Prussia, Pennsylvania

Daniel M. Zavisza

Hercules Incorporated Wilmington, Delaware

Randall W. Zempel

Dow Chemical Company Midland, Michigan

Ulrich Zorll

Forschungsinstitut fur Pigmente and Lacke

Stuttgart, Germany

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xi

Contents

I

Fundamentals and Testing

1 Rheology and Surface Chemistry ...1-1 K. B. Gilleo

2 Coating Rheology ...2-1 Chi-Ming Chan and Subbu Venkatraman

3 Leveling...3-1 D. Satas*

4 Structure–Property Relationships in Polymers ...4-1 Subbu Venkatraman

5 The Theory of Adhesion...5-1 Carl A. Dahlquist

6 Adhesion Testing...6-1 Ulrich Zorll

7 Coating Calculations ...7-1 Arthur A. Tracton

8 Infrared Spectroscopy of Coatings...8-1 Douglas S. Kendall

9 Thermal Analysis for Coatings Characterizations...9-1 William S. Gilman

10 Color Measurement for the Coatings Industry...10-1 Harold Van Aken

11 The Use of X-ray Fluorescence for Coat Weight Determinations ...11-1 Wayne E. Mozer

12 Sunlight, Ultraviolet, and Accelerated Weathering...12-1 Patrick Brennan and Carol Fedor

13 Cure Monitoring: Microdielectric Techniques ...13-1 David R. Day

14 Test Panels ...14-1 Douglas Grossman and Patrick Patton

*Deceased.

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xii

15 Design of Experiments for Coatings...15-1 Mark J. Anderson and Patrick J. Whitcomb

16 Top 10 Reasons Not to Base Service Life Predictions upon Accelerated Lab

Light Stability Tests...16-1 Eric T. Everett

17 Under What Regulation? ...17-1 Arthur A. Tracton

II

Coating and Processing Techniques

18 Wire-Wound Rod Coating ...18-1 Donald M. MacLeod

19 Slot Die Coating for Low Viscosity Fluids...19-1 Harry G. Lippert

20 Extrusion Coating with Acid Copolymers and Lonomers ...20-1 Donald L. Brebner

21 Porous Roll Coater...21-1 Frederic S. McIntyre

22 Rotary Screen Coating...22-1 F. A. Goossens 23 Screen Printing ...23-1 Timothy B. McSweeney 24 Flexography ...24-1 Richard Neumann 25 Ink-Jet Printing ...25-1 Naomi Luft Cameron

26 Electrodeposition of Polymers...26-1 George E. F. Brewer

27 Electroless Plating...27-1 A. Vakelis

28 The Electrolizing Thin, Dense, Chromium Process...28-1 Michael O’Mary

29 The Armoloy Chromium Process...29-1 Michael O’Mary

30 Sputtered Thin Film Coatings ...30-1 Brian E. Aufderheide

31 Vapor Deposition Coating Technologies ...31-1 Lindas Pranevicius

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xiii 32 Cathodic Arc Plasma Deposition ...32-1

H. Randhawa

33 Industrial Diamond and Diamondlike Films ...33-1 Arnold H. Deutchman and Robert J. Partyka

34 Tribological Synergistic Coatings...34-1 Walter Alina

35 Chemical Vapor Deposition ...35-1 Deepak G. Bhat

36 Solvent Vapor Emission Control ...36-1 Richard Rathmell

37 Surface Treatment of Plastics...37-1 William F. Harrington, Jr.

38 Flame Surface Treatment ...38-1 H. Thomas Lindland

39 Plasma Surface Treatment...39-1 Stephen L. Kaplan and Peter W. Rose

40 Surface Pretreatment of Polymer Webs by Fluorine...40-1 R. Milker and Artur Koch

41 Calendering of Magnetic Media ...41-1 John A. McClenathan

42 Embossing ...42-1 John A. Pasquale III

43 In-Mold Finishing...43-1 Robert W. Carpenter

44 HVLP: The Science of High-Volume, Low-Pressure Finishing ...44-1 Steve Stalker

45 A Practical Guide to High-Speed Dispersion ...45-1 Herman Hockmeyer

III

Materials

46 Acrylic Polymers ...46-1 Ronald A. Lombardi and James D. Gasper

47 Vinyl Ether Polymers...47-1 Helmut W. J. Müller

48 Poly(Styrene-Butadiene) ...48-1 Randall W. Zempel

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xiv

49 Liquid Polymers for Coatings...49-1 Robert D. Athey, Jr.

50 Polyesters ...50-1 H. F. Huber and D. Stoye

51 Alkyd Resins ...51-1 Krister Holmberg

52 The Polyurea Revolution: Protective Coatings for the 21st Century ...52-1 Bruce R. Baxter

53 Phenolic Resins ...53-1 Kenneth Bourlier

54 Coal Tar and Asphalt Coatings ...54-1 Henry R. Stoner

55 Vulcanizate Thermoplastic Elastomers...55-1 Charles P. Rader

56 Olefinic Thermoplastic Elastomers...56-1 Jesse Edenbaum

57 Ethylene Vinyl Alcohol Copolymer (EVOH) Resins ...57-1 R. H. Foster

58 Elastomeric Alloy Thermoplastic Elastomers ...58-1 Charles P. Rader

59 Polyvinyl Chloride and Its Copolymers in Plastisol Coatings ...59-1 Jesse Edenbaum

60 Polyvinyl Acetal Resins...60-1 Thomas P. Blomstrom 61 Polyimides ...61-1 B. H. Lee 62 Parylene Coating...62-1 William F. Beach 63 Nitrocellulose ...63-1 Daniel M. Zavisza

64 Soybean, Blood, and Casein Glues ...64-1 Alan Lambuth

65 Fish Gelatin and Fish Glue...65-1 Robert E. Norland

66 Waxes ...66-1 J. David Bower

67 Carboxymethylcellulose ...67-1 Richey M. Davis

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xv 68 Hydroxyethylcellulose ...68-1

Lisa A. Burmeister

69 Antistatic and Conductive Additives...69-1 B. Davis

70 Silane Adhesion Promoters...70-1 Edwin P. Plueddemann

71 Chromium Complexes ...71-1 J. Rufford Harrison

72 Nonmetallic Fatty Chemicals as Internal Mold Release Agents in Polymers ...72-1 Kim S. Percell, Harry H. Tomlinson, and Leonard E. Walp

73 Organic Peroxides...73-1 Peter A. Callais

74 Surfactants for Waterborne Coatings Applications...74-1 Samuel P. Morell

75 Surfactants, Dispersants, and Defoamers for the Coatings, Inks, and

Adhesives Industries ...75-1 John W Du

76 Pigment Dispersion ...76-1 Theodore G. Vernardakis

77 Colored Inorganic Pigments...77-1 Peter A. Lewis 78 Organic Pigments ...78-1 Peter A. Lewis 79 Amino Resins ...79-1 George D. Vaughn 80 Driers ...80-1 Milton Nowak

81 Biocides for the Coatings Industry ...81-1 K. Winkowski

82 Clays...82-1 Ashok Khokhani

83 Fluorocarbon Resins for Coatings and Inks...83-1 Kurt A. Wood

84 High Temperature Pigments...84-1 Helen Hatcher

85 Polyurethane Associative Thickeners for Waterborne Coatings ...85-1 Douglas N. Smith and Detlef van Peij

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xvi

IV

Surface Coatings

86 Flexographic Inks...86-1 Sam Gilbert 87 Multicolor Coatings...87-1 Robert D. Athey, Jr.

88 Paintings Conservation Varnish...88-1 Christopher W. McGlinchey

89 Thermoset Powder Coatings...89-1 Lawrence R. Waelde

90 Peelable Medical Coatings ...90-1 Donald A. Reinke

91 Conductive Coatings ...91-1 Raimond Liepins

92 Silicone Release Coatings ...92-1 Richard P. Eckberg

93 Silicone Hard Coatings...93-1 Edward A. Bernheim

94 Pressure-Sensitive Adhesives and Adhesive Products...94-1 D. Satas* 95 Self-Seal Adhesives...95-1 Larry S. Timm 96 Solgel Coatings...96-1 Lisa C. Klein 97 Radiation-Cured Coatings ...97-1 Joseph V. Koleske

98 Nonwoven Fabric Binders ...98-1 Albert G. Hoyle 99 Fire-Retardant/Fire-Resistive Coatings...99-1 Joseph Green 100 Leather Coatings ...100-1 Valentinas Rajeckas 101 Metal Coatings ...101-1 Robert D. Athey, Jr.

102 Corrosion and Its Control by Coatings ...102-1 Clive H. Hare

103 Marine Coatings Industry...103-1 Jack Hickey

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xvii 104 Decorative Surface Protection Products...104-1

Jaykumar (Jay) J. Shah

105 Coated Fabrics for Protective Clothing ...105-1 N. J. Abbott

106 Coated Fabrics for Apparel Use: The Problem of Comfort...106-1 N. J. Abbott

107 Architectural Fabrics ...107-1 Marcel Dery

108 Gummed Tape ...108-1 Milton C. Schmit

109 Transdermal Drug Delivery Systems ...109-1 Gary W. Cleary

110 Optical Fiber Coatings ...110-1 Kenneth Lawson

111 Exterior Wood Finishes ...111-1 William C. Feist

112 Pharmaceutical Tablet Coating...112-1 Joseph L. Johnson

113 Textiles for Coating...113-1 Algirdas Matukonis

114 Nonwovens as Coating and Laminating Substrates...114-1 Albert G. Hoyle

115 General Use of Inks and the Dyes Used to Make Them ...115-1 Carol D. Klein

116 Gravure Inks...116-1 Sam Gilbert

117 Artist’s Paints: Their Composition and History...117-1 Michael Iskowitz

118 Fade Resistance of Lithographic Inks — A New Path Forward: Real World Exposures in Florida and Arizona Compared to Accelerated Xenon Arc

Exposures...118-1 Eric T. Everett, John Lind, and John Stack

References

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