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Localization-induced coherent backscattering effect in wave dynamics

H. Schomerus, K. J. H. van Bemmel, and C. W. J. Beenakker

Instituut-Lorentz, Universiteit Leiden, P.O. Box 9506, 2300 RA Leiden, The Netherlands 共Received 1 September 2000; published 22 January 2001兲

We investigate the statistics of single-mode delay times of waves reflected from a disordered waveguide in the presence of wave localization. The distribution of delay times is qualitatively different from the distribution in the diffusive regime, and sensitive to coherent backscattering: The probability of finding small delay times is enhanced by a factor close to

2 for reflection angles near the angle of incidence. This dynamic effect of coherent backscattering disappears in the diffusive regime.

DOI: 10.1103/PhysRevE.63.026605 PACS number共s兲: 42.25.Dd, 42.25.Hz, 72.15.Rn

I. INTRODUCTION

The two most prominent interference effects arising from multiple scattering are coherent backscattering and wave lo-calization 关1–6兴. Both effects are related to the static inten-sity of a wave reflected or transmitted by a medium with randomly located scatterers. Coherent backscattering is the enhancement of the reflected intensity in a narrow cone around the angle of incidence, and is a result of the system-atic constructive interference in the presence of time-reversal symmetry关4,5兴. Localization arises from systematic destruc-tive interference, and suppresses the transmitted intensity关6兴. This paper presents a detailed theory of a recently discov-ered关7兴interplay between coherent backscattering and local-ization in a dynamic scattering property, the single-mode de-lay time of a wave reflected by a disordered waveguide. The single-mode delay time is the derivative ␾

d/d␻ of the phase␾of the wave amplitude with respect to the frequency ␻. It is linearly related to the Wigner-Smith delay times of scattering theory关8–10兴, and is the key observable of recent experiments on multiple scattering of microwaves 关11兴 and light waves 关12兴. Van Tiggelen, et al.关13兴developed a sta-tistical theory for the distribution of ␾

in a waveguide ge-ometry共where angles of incidence are discretized as modes兲. Although the theory was worked out mainly for the case of transmission, the implications for reflection are that the dis-tribution P(

) does not depend on whether the detected mode n is the same as the incident mode m or not. Hence it appears that no coherent backscattering effect exists for P(

).

What we will demonstrate here is that this is true only if wave localization may be disregarded. Previous studies 关11,13兴dealt with the diffusive regime of waveguide lengths L below the localization length␰.共The localization length in a waveguide geometry is ␰⯝Nl, with N the number of propagating modes and l the mean free path.兲Here we con-sider the localized regime L⬎␰ 共assuming that also the ab-sorption length␰a⬎␰). The distribution of reflected intensity

is insensitive to the presence or absence of localization, be-ing given in both regimes by Rayleigh’s law. In contrast, we find that the delay-time distribution changes markedly as one enters the localized regime, decaying more slowly for large 兩␾

兩. Moreover, a coherent backscattering effect appears: For L⬎␰ the peak of P(

) is higher for nm than for n

m by a factor which is close to

2, the precise factor being

2⫻(4096/1371␲)⫽1.35.

We also consider what happens if time-reversal symmetry is broken, by some magneto-optical effect. The coherent backscattering effect disappears. However, even for nm, the delay-time distribution for preserved time-reversal sym-metry is different than for broken time-reversal symsym-metry. This difference is again only present for L⬎␰, and vanishes in the diffusive regime.

The plan of this paper is as follows: In Sec. II we specify the notion关11兴of the single-mode delay time␾

, relate it to the Wigner-Smith delay times, and review the results 关13兴 for the diffusive regime, extending them to include ballistic corrections. This section also contains the random-matrix formulation for the localized regime, that provides the basis for our calculations, and includes a brief discussion of the conventional coherent backscattering effect in the static in-tensity I. Section III presents the calculation of the joint dis-tribution of␾

and I. We compare our analytical theory with numerical simulations, and give a qualitative argument for the dynamic coherent backscattering effect. The role of ab-sorption is discussed, as well as the effect of broken time-reversal symmetry. Details of the calculation are delegated to the Appendixes.

II. DELAY TIMES A. Single-mode delay times

We consider a disordered medium共mean free path l) in a waveguide geometry共length L), as depicted in Fig. 1. There are NⰇ1 propagating modes at frequency ␻, given by N ⫽␲A/␭2 for a waveguide with an opening of areaA. The wave velocity is c, and we consider a scalar wave共 disregard-ing polarization兲for simplicity. In the numerical simulations we will work with a two-dimensional waveguide of width W, where N2W/␭.

We study the dependence of the reflected wave amplitude

rnm

Iei␾ 共1兲

on the frequency␻. The indices n and m specify the detected and incident mode, respectively. 共We assume single-mode excitation and detection.兲 Here I⫽兩rnm兩2 is the intensity of

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intensity, and characterizes the static properties of the re-flected wave. Dynamic information is contained in the phase derivative

d

d␻, 共2兲

which has the dimension of a time and is called the single-mode delay time 关11,13兴. The intensity I and the delay time

can be recovered from the product of reflection matrix elements

␳⫽rnm共␻⫹

1

2␦␻兲rnm* 共␻⫺

1

2␦␻兲, 共3兲

evaluated at two nearby frequencies ␻⫾12␦␻. To leading

order in the frequency difference␦␻ one has

␳⫽I共1⫹i␦␻␾

兲⇒I⫽ lim ␦␻0

Re␳, ␾

⫽ lim ␦␻0

Im␳ ␦␻I.

共4兲

We seek the joint distribution function P(I,

) in an en-semble of different realizations of disorder. We distinguish between the diffusive regime where L is small compared to the localization length ␰⯝Nl, and the localized regime where Lⲏ␰. Localization also requires that the absorption length ␰aⲏ␰. We will contrast the case of excitation and

detection in two distinct modes nm with the equal-mode case nm. Although we mainly focus on the optically more relevant case of preserved time-reversal symmetry, we will also discuss the case of broken time-reversal symmetry for comparison. These two cases are indicated by the indexes ␤⫽1 and 2, respectively.

B. Relation to Wigner-Smith delay times

In the localized regime (␰ⰆL,a) we can relate the

single-mode delay time ␾

to the Wigner-Smith关8–10兴 de-lay times ␶i, with i1, . . . ,N. Thei’s are defined for a

unitary reflection matrix rcomposed of the elements rnm);

hence they require the absence of transmission and of ab-sorption. One then has

irdr d␻⫽U

diag␶1, . . . ,

NU, 共5a兲

ir*dr T

d␻⫽V

diag␶1, . . . ,

NV, 共5b兲

with U and V unitary matrices of eigenvectors. In the pres-ence of time-reversal symmetry r is a symmetric matrix; hence VU in this case.

For small ␦␻we can expand

r共␻⫾1

2␦␻兲⫽V

TU1 2i␦␻V

T diag␶1, . . . ,

NU. 共6兲

Inserting this into Eq. 共3兲and comparing with Eq.共4兲yields the relations

⫽ReA1 A0

, I⫽兩A0兩2, Ak

ii

ku

ivi. 共7兲

We have abbreviated uiUim and viVin. In the special

case nm, the coefficients ui and vi are identical in the

presence of time-reversal symmetry.

The distribution of the Wigner-Smith delay times in the localized regime was determined recently 关14兴. In terms of the rates ␮i⫽1/␶i it has the form of the Laguerre ensemble

of random-matrix theory,

P共兵␮i其兲⬀

ij 兩␮i⫺␮j兩 ␤

k ⌰共␮k

e⫺␥(␤N⫹2⫺␤)␮k,8

where the step function ⌰(x)1 for x0 and 0 for x⬍0. The parameter ␥ is defined by

␥⫽␣l/c, 共9兲

with the coefficient ␣⫽␲2/4 or 8/3 for two- or three-dimensional scattering, respectively. Equation 共8兲 extends the N⫽1 result of Refs.关15–17兴to any N.

The matrices U and V in Eq.共6兲are uniformly distributed in the unitary group. They are independent for ␤⫽2, while UV for ␤⫽1. In the large-N limit the matrix elements become independent Gaussian random numbers with vanish-ing mean and variance 1/N. Hence

ui

vi

⫽0,

具兩

ui兩2

vi兩2

N⫺1, 共10兲

with uivifor nm and␤⫽1. Corrections to this Gaussian

approximation are of order 1/N.

C. Diffusion theory

The joint probability distribution P(I,

) in the diffusive regime lLⰆ␰ was derived in Refs.关11,13兴,

Pdiff共I,

兲⫽⌰共I兲共I/¯I3兲1/2eI/ I

¯

Q¯

2兲⫺1/2

⫻exp

I I ¯

共␾

⫺␾¯

2

[image:2.612.57.296.61.170.2]

Q¯

2

, 共11兲

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with constants I¯,¯

, and Q. It has the same form for trans-mission and reflection, the only difference being the depen-dence of the constants on the system parameters. Here we focus on the case of reflection, because we are concerned with coherent backscattering.

From the joint distribution function 关Eq. 共11兲兴, for the intensity one obtains the Rayleigh distribution

Pdiff共I兲⫽ 1 I

¯exp共⫺I/ I¯兲. 共12兲

Hence I¯ is the mean detected intensity per mode. It is given by关18兴

I ¯1

N共1⫹␦␤1␦nm兲, 共13兲

assuming unit incident intensity. The factor of 2 enhance-ment in the case nm is the static coherent backscattering effect mentioned in Sec. I, which exists only in the presence of time-reversal symmetry (␤⫽1). Equations共12兲and共13兲 remain valid in the localized regime, since they are deter-mined by scattering on the scale of the mean free path. Hence Ll is sufficient for static coherent backscattering, and it does not matter whether L is small or large compared to␰.

By integrating over I in Eq.共11兲one arrives at the distri-bution of single-mode delay times关11,13兴,

Pdiff共␾

兲⫽ Q

2␾¯

Q⫹共␾

/␾

¯

12⫺3/2. 14

Hence␾¯

is the mean delay time, while

Q sets the relative width of the distribution. These constants are determined by the correlator 关11,13兴

C12⫽

rnm共␻⫹␦␻兲rnm* 共␻兲

rnm共␻兲rnm* 共␻兲

⫽1⫹i¯

␦␻⫺1

2␾¯

2Q1兲共␦␻2. 15

Diffusion theory gives

¯

2s/3, Q2s/5. 16

Here␥ is given by Eq.共9兲. We have defined

s⫽␣

L/l, 共17兲

where the numerical coefficient ␣

⫽2/␲, 3/4 for two- and three-dimensional scattering.共The corresponding result for Q given in Ref. 关13兴is incorrect.兲

Diffusion theory predicts that the distribution of delay times 关Eq. 共14兲兴, as well as the values of the constants ␾¯

and Q, do not depend on the choice nm or nm 共and also not on whether time-reversal symmetry is preserved or not兲. Hence there is no dynamic effect of coherent backscattering in the diffusive regime.

D. Ballistic corrections

The expressions for the constants I¯,¯

, and Q given above are valid up to corrections of order l/L. Here we give more accurate formulas that account for these ballistic cor-rections.共We need these to compare with numerical simula-tions.兲 We determine the ballistic corrections for Q and¯

by relating the dynamic problem to a static problem with absorption. 共This relationship only works for the mean. It cannot be used to obtain the distribution 关19兴.兲 The mean total reflectivity

a

¯1x

2xx2coths

2xx2arcosh1x兲兴 共18兲

for absorption␣

x per mean free path was evaluated in Ref. 关20兴.关Here␣

is the same constant as in the definition of s; see Eq. 共17兲.兴 We identify C12⫽¯ (x)/a¯(0) by analyticala continuation to an imaginary absorption rate x⫽⫺i␦␻␥. Expanding in x to second order, we find

¯

s共3⫹2s兲 3共1⫹s兲 , Q

8s3⫹28s2⫹30s⫹15 5共2s⫹3兲2 . 共19兲

E. Numerical simulation

The validity of diffusion theory was tested in Refs.关11– 13兴by comparison with experiments in transmission. In Fig. 2 we show an alternative test in reflection, by comparison with a numerical simulation of scattering of a scalar wave by a two-dimensional random medium. 共We assume time-reversal symmetry.兲The reflection matrices r(␻⫾1

2␦␻) are

computed by applying the method of recursive Green func-tions关21兴to the Helmholtz equation on a square lattice共 lat-tice constant a). The width W100 a and the frequency␻ ⫽1.4 c/a are chosen such that there are N⫽50 propagating modes. The mean free path l14.0 a is found from the for-mula关22兴tr rrNs(1s)⫺1 for the reflection probability. The corresponding localization length ␰⫽NL/s1100 a. The parameter␥⫽46.3 a/c is found from Eq.共19兲by

equat-FIG. 2. Distribution of the single-mode delay time ␾⬘ in the diffusive regime. The result of numerical simulation 共data points兲 with N⫽50 propagating modes is compared to the prediction关Eq.

共14兲兴 of diffusion theory共solid curve兲. There is no difference be-tween the case nm of equal-mode excitation and detection共open circles兲 and the case nm of excitation and detection in distinct

[image:3.612.354.520.57.174.2]
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ing

⫽␾¯

.共This value of␥ is somewhat larger than the value ␥⫽␲2l/4c34.5 a/c expected for two-dimensional scattering, as a consequence of the anisotropic dispersion relation on a square lattice.兲 We will use the same set of parameters later in this paper in the interpretation of the re-sults in the localized regime. Our numerical rere-sults confirm that in the diffusive regime the distribution of delay times␾

does not distinguish between excitation and detection in dis-tinct modes (nm, full circlesand identical modes (nm, open circles兲.

III. DYNAMIC COHERENT BACKSCATTERING EFFECT A. Distinct-mode excitation and detection

We now calculate the joint probability distribution func-tion P(I,

) of intensity I and single-mode delay time

in the localized regime, for the typical case nm of excitation and detection in two distinct modes. We assume a preserved time-reversal symmetry (␤⫽1), leaving the case of broken time-reversal symmetry for the end of this section.

It is convenient to work momentarily with the weighted delay time W⫽␾

I and to recover P(I,

) from P(I,W) at the end. The characteristic function

␹共p,q兲⫽

ei pIiqW

共20兲

is the Fourier transform of P(I,W). The average

•••

is over the vectors u and v and over the set of eigenvalues兵␶i其.

The average over one of the vectors, say v, is easily carried out, because it is a Gaussian integration. The result is a de-terminant:

␹共p,q兲⫽

det共1⫹iH/N兲⫺1

, 共21a兲

Hpu*uT⫹1 2q*u

Tu*¯uT. 21b

The Hermitian matrix H is a sum of dyadic products of the vectors u and u¯, with u¯iuii, and hence has only two non-vanishing eigenvalues ␭ and ␭. Some straightfor-ward linear algebra gives

⫽1

2共qB1⫹p

2 pqB1⫹q2B2⫹p2兲, 共22兲 where we have defined the spectral moments

Bk

i

ui兩2␶i

k. 23

The resulting determinant is

det共1⫹H/N兲⫺1⫽共1⫹␭/N兲⫺1共1⫹␭/N兲⫺1; 共24兲

hence

␹共p,q兲⫽

1⫹i p N

iq

NB1⫹ q2

4N2共B2⫺B1 2

⫺1

. 共25兲

An inverse Fourier transform, followed by a change of vari-ables from I,W to I,

, gives

PI,

兲⫽⌰共I兲共N3I/␲兲1/2eNI

B2⫺B1

21/2exp

NI共␾

B1兲 2

B2⫺B1 2

.

共26兲

The average is over the spectral moments B1 and B2, which depend on the ui’s and ␶i’s via Eq. 共23兲.

The calculation of the joint distribution P(B1,B2) is pre-sented in Appendix A. The result is

PB1,B2兲⫽⌰共B1兲⌰共B2兲exp

NB12

B2

B1 2

N3

B24 共B2⫹␥N 2B

1兲exp

⫺ 2␥N

B1

⫺␥ 3N5

4B25 共2B2 24B

1 2B

2NB1

4N2Ei

2␥N B1

,

共27兲

where Ei(x) is the exponential-integral function. The distri-bution P(I,

) follows from Eq.共26兲by integrating over B1 and B2 with weight given by Eq.共27兲.

Irrespective of the distribution of B1 and B2, from Eq. 共26兲we recover the Rayleigh law关Eq.共12兲兴for the intensity I. The distribution P(

)⫽兰0d I P(I,

) of the single-mode delay time takes the form

P共␾

兲⫽

0

dB1

0

dB2

PB1,B2兲共B2⫺B1 2

2共B2⫹␾

2⫺2B1␾

兲3/2 . 共28兲

[image:4.612.351.523.57.178.2]

In Fig. 3 this distribution is compared with the result of a numerical simulation of a random medium as in Sec. II E, but now in the localized regime. The same value for ␥ was used as in Fig. 2, making this comparison a parameter-free test of the theory.共Note that␥alone determines the complete distribution function in the localized regime, in contrast to

FIG. 3. Distribution of the single-mode delay time ␾⬘ in the localized regime. The results of numerical simulations with N

⫽50 propagating modes共open circles for nm, full circles for n

m) are compared to the analytical predictions. The curve for

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the diffusive case where two parameters are required.兲The numerical data agree very well with the analytical prediction.

B. Equal-mode excitation and detection

We now turn to the case nm of equal-mode excitation and detection, still assuming that time-reversal symmetry is preserved. Since uivi, we now have

⫽ReC1 C0

, I⫽兩C0兩2, Ck

ii

ku i

2. 29

The joint distribution function P(C0,C1) of these complex numbers can be calculated in the same way as P(B1,B2). In Appendix C we obtain

PC0,C1兲⬀exp共⫺NC0兩2/2兲

0

dss2es

1⫹兩C1兩 2s2

␥2N2 ⫺ 2s

NRe C0C1*

⫺5/2 . 共30兲

The corresponding distribution function P(

) is also plot-ted in Fig. 3, and compared with the results of the numerical simulation. Good agreement is obtained, without any free parameter.

C. Comparison of both situations

Comparing the two curves in Fig. 3, we find a striking difference between distinct-mode and equal-mode excitation and detection: The distribution for nm displays an en-hanced probability of small delay times. In the vicinity of the peak, both distributions become very similar when the delay times for nm are divided by a scale factor of about

2. In the limit N→⬁ 共see Sec. III D兲, the maximal value P(␾peak

)⫽

2/␲N3␥2 for nm is larger than the maximum of P(

) for nm by a factor

Pnm共␾peak

Pnm共␾peak

2⫻ 4096

1371␲⫽1.35. 共31兲

Correspondingly, the probability to find very large delay times is reduced for nm. This is reflected by the asymptotic behavior

P共␾

兲⬃␥N 3/2

2

共2␲兲⫺1/2 for nm

冑␲

/4 for nm. 共32兲

The enhanced probability of small delay times for nm is the dynamic coherent backscattering effect mentioned in Sec. I. The effect requires localization, and is not observed in the diffusive regime.

D. Limit N\

The results presented so far assume NⰇ1, but retain finite-N corrections of order N⫺1/2.共Only terms of order 1/N and higher are neglected.兲It turns out that the asymmetry of

P(

) for positive and negative values of␾

is an effect of order N⫺1/2. The asymmetry is hence captured faithfully by our calculation. We now consider how the asymmetry even-tually disappears in the limit N→⬁.

For distinct modes nm, the spectral moments scale as B1⬃␥N and B2⬃␥2N3. With␾

⬃␥N3/2, one finds that B1 can be omitted to order N⫺1/2 in Eq.共28兲. One obtains the symmetric distribution

P共␾

兲⫽

0

dB2

PB2B2

2共B2⫹␾

23/2 共33兲

plotted in Fig. 4.

For identical modes nm, observe that the quantities C0 and C1 become mutually independent in the large-N limit: The cross-term (␥N)⫺1 Re C0C1* in Eq. 共30兲 is of relative order N⫺1/2 because C0⬃N⫺1/2 and C1⬃␥N. Hence, to or-der N⫺1/2, the distribution factorizes, P(C0,C1) ⫽P(C0) P(C1). The distribution of C0 is a Gaussian,

PC0兲⫽ N

2␲exp共⫺NC0兩

2/2, 34

as a consequence of the central-limit theorem, and

PC1兲⬀

0

dss2es

1⫹兩C1兩 2s2

␥2N2

⫺5/2

. 共35兲

The resulting distribution of ␾

Re(C1/C0) is also plotted in Fig. 4.

[image:5.612.356.522.56.176.2]

The dynamic coherent backscattering effect persists in the limit N→, it is therefore not due to finite-N corrections. The peak heights differ by the factor given in Eq. 共31兲.

FIG. 4. Distribution of the single-mode delay time ␾⬘ in the localized regime for preserved time-reversal symmetry, in the limit

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E. Interpretation in terms of large fluctuations In order to explain the coherent backscattering enhance-ment of the peak of P(

) in more qualitative terms, we compare Eq. 共29兲for nm with the corresponding relation 关Eq. 共7兲兴for nm.

The factorization of the joint distribution function P(C0,C1) discussed in Sec. III D can be seen as a conse-quence of the high density of anomalously large Wigner-Smith delay times␶iin the Laguerre ensemble关Eq.共8兲兴. The

distribution of the largest time␶max⫽maxiifollows from the

distribution of the smallest eigenvalue in the Laguerre en-semble, calculated by Edelman关23兴. It is given by

P共␶max兲⫽␥N 2

␶max2 exp共⫺␥N

2/␶max. 36

As a consequence, the spectral moment C1is dominated by a small number of contributions ui2␶i共often enough by a single

one, say with index i1), while C0 can be safely approxi-mated by the sum over all remaining indices isay, i⫽1). The same argument applies also to the spectral moments Ak

which determine the delay-time statistics for nm; hence the distribution function P(A0,A1) factorizes as well.

The quantities A0 and C0have a Gaussian distribution for large N, because of the central-limit theorem, with P(C0) given by Eq.共34兲and

PA0兲⫽N

␲exp共⫺NA0兩2兲. 共37兲

It then becomes clear that the main contribution to the en-hancement关Eq. 共31兲兴of the peak height, namely, the factor of

2, has the same origin as the factor of 2 enhancement of the mean intensity I¯. More precisely, the relation P(A0⫽x)2 P(C0⫽

2x) leads to a rescaling of P(I) for nm by a factor of 1/2 and to a rescaling of P(

) by a factor of

2. The remaining factor of 4096/1371␲⫽0.95 comes from the difference in the distributions P(A1) and P(C1). It turns out that the distribution

PA1兲⫽

0

ds 1

4␲␥N

s2

共4⫹兩A1/␥N兩2s2兲3

⫻关es共64⫹32s12s2⫹s3兲⫺3s2 Ei共⫺s兲兴 共38兲

共derived in Appendix D兲is very similar to P(C1) given in Eq. 共35兲; hence the remaining factor is close to unity.

The large ␶i’s are related to the penetration of the wave

deep into the localized regions and are eliminated in the dif-fusive regime Lⱗ␰. In Sec. III F we compare the localized and diffusive regimes in more detail.

F. Localized vs diffusive regime

Comparison of Eqs.共11兲and共26兲shows that the two joint distributions of I and

would be identical if statistical fluc-tuations in the spectral moments B1and B2could be ignored. The correspondences are

B1¯

, B2⫺B1

2Q¯

2. 39

However, the distribution P(B1,B2) is very broad 共see Fig. 5兲, so that fluctuations cannot be ignored. The most probable values are

B1typical⯝␥N, B2typical⯝␥2N3, 共40兲

but the mean values

B1典,

B2典 diverge—demonstrating the presence of large fluctuations. In the diffusive regime Lⱗ␰ the spectral moments B1 and B2 can be replaced by their ensemble averages, and the diffusion theory关11,13兴is recov-ered. 共The same applies if the absorption length␰aⱗ␰.兲

The large fluctuations in B1 and B2 directly affect the statistical properties of the delay time ␾

. We compare the distribution 关Eq. 共28兲兴 in the localized regime 共Fig. 3兲 with the result关Eq.共14兲兴of diffusion theory共Fig. 2兲. In the local-ized regime the value␾peak

B1typicalat the center of the peak of P(

) is much smaller than the width of the peak⌬␾

(B2typical)1/2⯝␾peak

(␰/l)1/2. This also holds in the diffusive regime, where␾peak

⫽␾¯

and⌬␾

⯝␾peak

(L/l)1/2. However, the mean

具␾

B1典 diverges for P, but is finite共equal to ␾¯

) for Pdiff. For large B2 one has, asymptotically, P(B2) ⬃1

4N

3/2

冑␲

B 2

⫺3/2

. As a consequence, in the tails P(

) falls off only quadratically关see Eq.共32兲兴, while in the diffu-sive regime Pdiff(␾

)⬃

1 2Q¯

2兩␾

⫺3 falls off with an in-verse third power.

G. Role of absorption

[image:6.612.352.524.56.180.2]

Although absorption causes the same exponential decay of the transmitted intensity as localization, this decay is of a quite different, namely, an incoherent, nature. The strong fluctuations in the localized regime disappear as soon as the absorption length ␰a drops below the localization length␰, because long paths which penetrate into the localized regions

FIG. 5. Distributions of B˜1⫽B1/␥N and B˜2⫽B2/␥2N3. The

analytic prediction from Eq. 共27兲 关for explicit formulas see Eqs.

(7)

are suppressed by absorption. In this situation one should expect that the results of diffusion theory are again valid even for Lⲏ␰. This expectation is confirmed by our numeri-cal simulations.共We do not know how to incorporate absorp-tion effects into our analytical theory.兲

In Fig. 6 we plot the delay-time distribution for two val-ues of the absorption length␰a⬍␰and one value␰a⬎␰, both

for equal-mode and distinct-mode excitation and detection. The length of the waveguide is L⫽4.1␰. The result for strong absorption with ␰a⫽0.11␰ is very similar to Fig. 2.

Irrespective of the choice of the detection mode, the data can be fitted to prediction 共14兲of diffusion theory. The plot for ␰a⫽0.47␰ shows that the dynamic coherent backscattering

effect slowly sets in when the absorption length becomes comparable to the localization length. The data also deviate from the prediction of diffusion theory. The full factor关Eq. 共31兲兴 between the peak heights quickly develops as soon as

a exceeds ␰, as can be seen from the data for ␰a⫽2.1␰.

Moreover, these data can already be fitted to the predictions of random-matrix theory, with ␥⬇53.2 a/c. 共The value ␥ ⫽46.3 a/c of Sec. II E is reached when absorption is further reduced.兲

H. Broken time-reversal symmetry

The case ␤⫽2 of broken time-reversal symmetry is less important for optical applications, but has been realized in microwave experiments关24–26兴. There is now no difference between nm and nm. The matrices U and V have the same statistical distribution as for the case of preserved time-reversal symmetry. Hence, by following the steps of Sec. III A, we arrive again at Eq. 共26兲, with spectral moments Bk

as defined in Eq.共23兲. Their joint distribution has now to be calculated from Eq.共8兲with␤⫽2. This calculation is carried out in Appendix B. The result is

PB1,B2兲⫽2␥N 3B

1 2

B23 exp共⫺NB1 2/B

2⫺2␥N/B1兲. 共41兲

The distribution of single-mode delay times P(

) is given by Eq.共28兲, with the function P(B1,B2). We plot P(

) in Fig. 7, and compare it to the case of preserved time-reversal symmetry. The distribution is rescaled by about a factor of 2 toward larger delay times when time-reversal symmetry is broken. This can be understood from the fact that the rel-evant length scale, the localization length, is twice as large for broken time-reversal symmetry (␰⫽2NL/s, while ␰ ⫽NL/s for preserved time-reversal symmetry兲.

IV. CONCLUSION

[image:7.612.78.267.56.430.2]

We have presented a detailed theory, supported by nu-merical simulations, of a recently discovered 关7兴 coherent backscattering effect in the single-mode delay times of a wave reflected by a disordered waveguide. This dynamic ef-fect is special because it requires localization for its exis-tence, in contrast to the static coherent backscattering effect in the reflected intensity. The dynamic effect can be under-stood from the combination of the static effect and the large

FIG. 6. Single-mode delay-time distribution P(␾⬘) in the pres-ence of absorption. The data points are the result of a numerical simulation of a waveguide with length L⫽4.5␰. Open circles are for equal-mode excitation and detection nm, and full circles for the

case of distinct modes nm. In the upper panel 共with␰a⬍␰), the

data are compared to the prediction关Eq.共14兲兴of diffusion theory. In the lower panel we compare with the predictions 关Eqs. 共27兲–

[image:7.612.355.521.56.178.2]

共30兲兴of random-matrix theory.

FIG. 7. Comparison of the single-mode delay-time distributions for preserved and broken time-reversal symmetry. The number of propagating modes is N⫽50. The curves are calculated from Eq.

共28兲, with P(B1,B2) given by Eq. 共27兲 (␤⫽1) or Eq. 共41兲 (␤

(8)

fluctuations in the localized regime.

In the diffusive regime there is no dynamic coherent backscattering effect: The distribution of delay times is un-affected by the choice of the detection mode and the pres-ence or abspres-ence of time-reversal symmetry. The effect also disappears when the absorption length is smaller than the localization length. In both situations the large fluctuations characteristic of the localized regime are suppressed.

Existing experiments on the delay-time distribution 关11,12兴verified the diffusion theory关13兴. The theory for the localized regime presented here awaits experimental verifi-cation.

ACKNOWLEDGMENTS

We thank P. W. Brouwer for valuable advice. This work was supported by the ‘‘Nederlandse organisatie voor Weten-schappelijk Onderzoek’’共NWO兲and by the ‘‘Stichting voor Fundamenteel Onderzoek der Materie’’共FOM兲.

APPENDIX A: JOINT DISTRIBUTION OF B1AND B2FORÄ1

We calculate the joint probability distribution function P(B1,B2) of the spectral moments B1and B2, defined in Eq. 共23兲, which determine P(I,

) from Eq. 共26兲. We assume preserved time-reversal symmetry (␤⫽1). Since Bk ⫽兺iui兩2␮i

k

, we have to average over the wave function amplitudes ui, which are Gaussian complex numbers with

zero mean and variance 1/N, and the ratesi which are

distributed according to the Laguerre ensemble关Eq.共8兲兴with ␤⫽1. This Laguerre ensemble is represented as the eigen-values of an NN Hermitian matrix WW, where W is a complex symmetric matrix with the Gaussian distribution:

PW兲⬀exp关⫺␥共N⫹1兲tr WW兴. 共A1兲

The calculation is performed neglecting corrections of order 1/N, so that we are allowed to replace N1 by N. The mea-sure is

dW

ij

d Re Wi jd Im Wi j

i

d Re Wiid Im Wii. 共A2兲

1. Characteristic function

In the first step we express P(B1,B2) by its characteristic function,

PB1,B2兲⫽ 1 共2␲兲2

⫺⬁

d p

⫺⬁ ⬁

dqei pB1⫹iqB2␹共p,q,

共A3兲

␹共p,q兲⫽

l1

N

exp

iul兩2

pl

q

l

2

, 共A4兲 and average over the ul’s:

␹共p,q兲⫽

l⫽1

N

1⫹i plN

i ql

2N

⫺1

det共W

W2

det关共WW兲2⫹i pWW/Niq/N

. 共A5兲

We have expressed the product over eigenvalues as a ratio of determinants. We write the determinant in the denominator as an integral over a complex vector z:

␹共p,q兲⬀

dW

dz exp关⫺␥N tr WW兴det共WW兲2 ⫻exp兵⫺z†关共WW兲2⫹i pWW/Niq/Nz其.

共A6兲

This integral converges because WW is positive definite.

2. Parametrization of the matrix W

Now we choose a parametrization of W which facilitates a stepwise integration over its degrees of freedom. The distri-bution of W is invariant under transformations W→UTWU, with any unitary matrix U. Hence we can choose a basis in which z points in direction 1, and write W in block form:

W

a xT

x X

. 共A7兲

Here a is a complex number. For any (N⫺1)-dimensional vector x we can use another unitary transformation on the X block after which x points in direction 2. Then W is of the form

W

a x 0T x b yT

0 y Y

, 共A8兲

with the real number x⫽兩x兩. In this parametrization

WW

11⫽兩a兩2⫹x2, 关共WW2

11⫽共兩a兩2⫹x2兲2⫹x2y2⫹x2兩ab*兩2, det W⫽关abyTY⫺1y兲⫺x2det Y ,

tr WWa2b22x22y2tr Y ,

d Wd2a d2bdx dy dY ,

with y⫽兩y. A suitable transformation on Y allows one to replace the term yTY⫺1y by y2(Y⫺1)

11.

For this parametrization of W, the integrand in Eq. 共A6兲 depends on the vectors x, y, and z only by their magnitudes x, y, and z⫽兩z. Hence we can replace dx→x2N⫺3dx, dy

(9)

3. Integration

The integrand in Eq.共A6兲involves z, p, and q in the form

exp†⫺z2共关共WW兲2兴11⫹i pWW兲11/Niq/N兲‡. 共A9兲

It is convenient to pass back to P(B1,B2) by Eq.共A3兲, be-cause integration over p and q gives delta functions: ␦关B1⫺z2共兩a兩2⫹x2兲/N兴␦共B2⫺z2/N

B1 2␦共

B1/B2⫺兩a兩2⫺x2兲␦共B2⫺z2/N兲. 共A10兲

Subsequent integration over z results in

PB1,B2兲⬀

d2ad2bdxdy x2N⫺3y2N⫺5B2

N⫺2

⫻共B1/B2⫺兩a兩2⫺x2兲关c0

⫻兩abx2兩4⫹4c2兩a兩2y4兩abx2兩2⫹c4兩a兩4y8兴

⫻exp

NB2

B1 2

B22⫹x

2y2x2a*⫹b2

⫺2␥Ny2

. 共A11兲

Here we omitted a term ␥N(a兩2⫹兩b兩2⫹2x2) in the expo-nent, because it is of order 1/N, as we shall see later. Fur-thermore, we denoted

cm

det Y兩4兩共Y⫺1兲11兩m

det Y兩4

. 共A12兲

These coefficients will be calculated later, with the results c0⫽1, c2⫽2␥, and c4⫽4␥2. Integration over y yields for the terms proportional to cm the factors (B2x2 ⫹2␥)⫺mN⫹2, which can be combined with the factor (B2x2)N⫺2, giving, to order 1/N 关we anticipate ␥/B2x2 ⫽O(1/N)兴,

B2x2兲N⫺2

B2x2⫹2␥兲N⫺2⫹m→B2x

2mexp

2␥N

B2x2

. 共A13兲

We introduce a new integration variable by b

ba*. So far P(B1,B2) is reduced to the form

PB1,B2兲⬀

d2ad2b

dxx␦共B1/B2⫺兩a兩2⫺x2兲 ⫻

ab

B1

B2

4

4c2兩a兩 2

B22x4

ab

B1 B2

2 ⫹c4兩a

4

B24x8

⫻exp

⫺2␥N

x2B 2

NB1 2

B2⫺

NB2x2兩b

兩2

. 共A14兲

Let us now convince ourselves with this expression that we were justified in omitting the term ␥N(a兩2⫹兩b兩2⫹2x2) in Eq.共A11兲and in using Eq.共A13兲. Indeed, the various quan-tities scale as B1⯝␥N, B2⯝␥2N3, and 兩a兩2⯝兩b兩2⯝x2 ⯝1/␥N2, because any␥ and N dependence disappears if one passes to appropriately rescaled quantities B1/␥N, etc. The terms omitted are therefore of order 1/N.

The remaining integrations in Eq. 共A14兲 are readily per-formed, with the final result Eq.共27兲. The distribution of B1, to order 1/N, is

PB1兲⫽ ␥N

B13共B1⫹2␥N兲exp

⫺ 2␥N

B1

. 共A15兲

The spectral moment B1 appeared before in a different physical context in Ref. 关20兴, but only a heuristic approxi-mation was given in that paper. Equation 共A15兲 solves this random-matrix problem precisely.

For completeness we also give the distribution of the other spectral moment B2 共rescaled as B˜2⫽B2␥⫺2N⫺3) in terms of Meijer G functions:

P2兲⫽ 1

64B˜25/2␲1/2

14␲B ˜216 G

3,0 0,3B˜2兩1

2,0, 3 2兲

20 G3,00,3共2兩⫺12, 1

2,1兲⫹22 G3,0 0,3

2兩12, 1 2,1兲

8 G3,00,3共2兩12,1, 3

2兲⫹4 G3,0 0,3

B ˜2兩1

2, 3 2,2兲

8 G4,11,3

2

⫺1

2,0, 3 2,2

1

16 G4,1 1,3

B ˜2

0,

1 2,

3 2,2

1

3 G4,10,4

2

1 2,

1 2,

3 2,

3 2

0

冊册

. 共A16兲

4. Coefficients

Now we calculate the coefficients c2and c4defined in Eq. 共A12兲. It is convenient to resize the matrix Y to dimension Ninstead of N⫺2), and to set␥N⫽1 momentarily. We again use a block decomposition,

Y

a wT

w Z

, 共A17兲

and employ the identities

det Y⫽共awTZ⫺1wdet Z, 共A18a兲

Y⫺1兲11⫽共awTZ⫺1w兲⫺1. 共A18b兲

Hence

c4⫽

具兩

det Z兩4

det Y兩4

4

N⫹1兲共N⫹3兲, 共A19兲

(10)

det Y兩4

⫽1 6

⌫共N⫹4兲⌫共N⫹2兲

22N . 共A20兲

In order to evaluate

c2

det Z

4a2wTZ⫺1w2

det Y兩4

, 共A21兲

it is again profitable to use unitary invariance and turn w in direction 1:

wTZ⫺1w兩2⫽w4兩共Z⫺1兲11兩2. 共A22兲

From

w4

⫽14N(N⫹1) and

具兩

a

2

1 we then obtain the recursion relation

c2共N兲⫽

4

N⫹1兲共N⫹3兲⫹ N

N⫹3c2共N⫺1兲, 共A23兲

which is solved by

c2共N兲⫽ 2

N⫹1. 共A24兲

In order to reintroduce␥we have to multiply cmby (␥N)m/2,

and obtain, to order 1/N,

c2⫽2␥, c4⫽4␥2, A25

as advertised above.

APPENDIX B: JOINT DISTRIBUTION OF B1AND B2FORÄ2

For broken time-reversal symmetry, the distributions of B1and B2have to be calculated from the Laguerre ensemble 关Eq.共8兲兴with␤⫽2. Similarly as for preserved time-reversal symmetry, this ensemble can be obtained from the eigenval-ues of a matrix WW. The matrix W is once more complex, but no longer symmetric 共it is also not Hermitian兲. It has a Gaussian distribution

PW兲⬀exp共⫺2␥N tr WW兲, 共B1兲

with measure

d W

i, j

d Re Wi jd Im Wi j. 共B2兲

It is instructive to calculate P(B1) first, because it will be instrumental in the calculation of P(B1,B2). After averaging over the ui’s, the characteristic function takes the form

␹共p兲⫽

exp共⫺i pB1兲

det WW

det共WWi p/N

. 共B3兲 We express the determinant in the denominator as an integral over a complex vector z. Due to the invariance W→UWV of P(W) for arbitrary unitary matrices U and V, we can turn z in direction 1, and write

W

a x

0T x

Y

0

. 共B4兲

Then

PB1兲⬀

d pdzz2N⫺1d2adxx2N⫺3dx

x

2N⫺3

⫻共兩a兩2⫹d2x2x

2兲exp关⫺共z2⫹2␥N兲共兩a兩2⫹x2兲兴 ⫻exp关i pB1z2/N兲⫺2␥Nx

2兴. 共B5兲

Selberg’s integral 关27兴gives

d2

具兩

det Y

2Y⫺111兩2

det Y兩2

⫽ 2␥N

N⫺1. 共B6兲

The integration over p gives(z2NB

1), and allows one to eliminate z. The integration over x

amounts to replacing x

2⫽(N⫺1)/2␥Nd2⫺1. The final integrations are most easily carried out by concatenating a to x, giving an N-dimensional vector y. Then

PB1兲⬀

dy y2N⫹1B1

N⫺1

⫻exp关⫺NB1⫹2␥兲y2兴 ⬀B1

N⫺1

B1⫹2␥兲⫺N⫺1, 共B7兲

which to order 1/N becomes

PB1兲⫽ 2␥N

B1

2 exp共⫺2␥N/B1兲. 共B8兲

The first steps in the calculation of the joint distribution function of B1 and B2 are identical to what was done in Appendix A, and result in the characteristic function␹( p,q) in the form of Eq.共A6兲, but with␥ replaced by 2␥. Due to the unitary invariance of the W ensemble we can write

W

a x

0 0T x b y

0T

0 y

Y

0 0

. 共B9兲

One now integrates over p and q and obtains delta functions as in Eq.共A10兲. This is followed by integration over z. The calculation is then much simplified by recognizing that one can rescale the remaining integration variables in such a way 共namely, by introducing a2⫽˜a2B1/B2, x2⫽˜x2B1/B2, y

2 ⫽˜y

2x⫺2B

2

⫺1) that

PB1,B2兲⫽B2⫺

3exp共⫺NB 1 2/B

(11)

It is not necessary here to give f (B1) as a lengthy multidi-mensional integral, since its functional form is easily recov-ered from the relation

PB1兲⫽

dB2PB1,B2兲⫽N⫺2B1⫺ 4

fB1兲. 共B11兲

We compare this with Eq. 共B8兲, and arrive at Eq.共41兲. The distribution of B2 has the closed-form expression

PB2兲⫽␥⫺2N⫺3G3,00,3共␥⫺2N⫺3B2兩⫺1

2,⫺1,⫺2兲.

共B12兲

APPENDIX C: JOINT DISTRIBUTION OF C0AND C1 We seek the joint distributions of the spectral moments C0 and C1, which determine ␾

and I for ␤⫽1 and nm via Eq.共29兲. We start with the characteristic function

␹共p0, p1兲⫽

exp关i Rep0C0⫹p1C1兲兴

, 共C1兲

where p0and p1 are complex numbers, as are the quantities C0and C1themselves. Since Ck⫽兺iui

2

i k

, we have to aver-age over the␶i’s and the ui’s. Averaging over the ui’s first,

we obtain

␹共p0, p1兲⫽

i

1⫹兩p1␶ip0兩 2

N2

⫺1/2

. 共C2兲 We again regard the rates ␮i⫽␶i

1

as the eigenvalues of a matrix product Y Y, where Y will be specified below. Then the product of square roots can be written as a ratio of de-terminants:

i

1⫹兩p1␶ip0兩 2

N2

⫺1/2

det Y YT det

Y YT兲2N 2p0兩2

N2

⫹2Re p0p1 *

N2 Y Y

Tp1兩

2

N2

⫺1/2

. 共C3兲

We will express the determinant in the denominator as a Gaussian integral over a real N-dimensional vector z. Hence it is convenient to choose Y real as well, so that one can use orthogonal invariance in order to turn z in direction 1. More-over, there is a representation of Y which allows one to in-corporate the determinant in the numerator into the probabil-ity measure: We take Y as a rectangular N(N⫹3) matrix with random Gaussian variables, distributed according to

PY兲⬀exp共⫺␥N tr Y YT兲. 共C4兲

The corresponding distribution of the eigenvalues␮iof Y YT is given in Ref.关23兴, and differs from the Laguerre ensemble 关Eq.共8兲兴by the additional factor兿iidet Y YT. In this

rep-resentation,

␹⬀

dzzN⫺1

exp兵⫺z2共1⫹兩p0兩2/N2兲关共Y YT兲2兴11其 ⫻exp

2 Re p0p1

*

N2 关Y Y T

11⫹ 兩p1兩2

N2

, 共C5兲 where the average is now over Y. Inverse Fourier transfor-mation with respect to p0 and p1 results in

PC0,C1兲⬀

dzzN⫺5 exp关⫺z

2关共Y YT2 11兴 关共Y YT兲2兴11⫺共关Y YT兴11兲2

⫻exp

⫺兩C1兩 2N2

4z2 ⫺ N2

4z2

⫻ 兩C0⫺关Y YT兴11C1兩2 关共Y YT兲2兴11⫺共关Y YT兴11兲2

. 共C6兲

The orthogonal invariance of Y YT allows us to param-etrize Y as

Y

a v 0T w b

0 y Z

0 0

, 共C7兲

with real numbers v0, w0, y0, a, and b, and an(N⫺1)⫻(N⫹1)兴-dimensional matrix Z. It is good to see that Z drops out of the calculation, because it does not appear in

Y YT兴11⫽a2⫹v2, 共C8a兲

关共Y YT兲2兴11⫽共a2⫹v2兲2⫹共awvb兲2⫹v2y2. 共C8b兲

We replace bb

aw/v, and introduce z

z yv. The inte-gral over z

can be written in the saddle-point form 兰dz

z

Nez⬘2f (z

)⬀f (

N/2) for large N. The resulting ex-pression varies with respect to the remaining variables on the scales

N3a2⯝N2b

2⯝N2v2N y2w2O⫺1. C9

(12)

PC0,C1兲⬀

dadb

dvv3dwwN⫺2dy y exp关⫺N y2 ⫻exp

⫺␥Nw2

1⫹a

2

v2

N

2 y2共v

2y2b

2

⫻exp

Nv2Re C0C1*⫺

Nv2y2兩C1兩2

2 ⫺

NC0兩2

2

. 共C10兲

Now we can integrate over a, b

, w, andv, and arrive at

PC0,C1兲⬀

d y

exp关⫺␥N y2⫺NC0兩2/2兴 共y⫺2⫹y2兩C1兩2⫹2 Re C0C1*兲

5/2. 共C11兲

The final result 关Eq. 共30兲兴 is obtained by substituting s ⫽␥Ny2.

APPENDIX D: DISTRIBUTION OF A1FORÄ1 In the large-N limit the joint distribution function P(A0,A1)⫽P(A0) P(A1) factorizes, as explained in Sec. III E. The distribution of A0 is given in Eq.共37兲. It remains to calculate the distribution of A1⫽兺iiuivi. The ui’s and

vi’s are independent Gaussian random numbers. Averaging

over them, we obtain the characteristic function

␹共p兲⫽

exp关i RepA1兲兴

i

1⫹兩pi兩 2

4N2

⫺1

det共W

W2

det关共WW兲2⫹兩p兩2/4N

, 共D1兲 where p is a complex number. The Laguerre ensemble is again represented as the eigenvalues of the matrix product WW, where W is the complex symmetric matrix with dis-tribution共A1兲. Following the route of Appendix A we rep-resent the determinant in the denominator by a Gaussian in-tegral over a complex vector z, and choose a basis in which W is of the form of Eq.共A8兲. The characteristic function is then obtained as the following multidimensional integral:

␹共p兲⫽

dx dy dz d2ad2bdYdet Y4aby2Y⫺1 11兴2

x2兩4exp

⫺兩z p兩 2

4N2

exp关⫺z

2„共a2x22x2a

b*兩2x2y2…兴exp关⫺Na2b2

2x22 y2tr YY兲兴. D2

Let us briefly describe in which order the integrations are performed most conveniently. Fourier transformation with respect to p converts the characteristic function back into the distribution function P(A1). This step gives rise to a factor z⫺2 exp(⫺兩A1兩2N2z⫺2). We can also integrate over y, which results in a factor exp关⫺2␥N/(xz)2兴. We introduce new vari-ables by the substitutions ba*, xv/z, and aa

/z. After these transformations one succeeds in integrating over b

, z, and a

. The remaining integral over v⫽兩v兩 is of the form

PA1兲⬀兩A1兩⫺5

dvv⫺5e⫺2/v

␲关8兩A1兩2共2⫹4vv2兲⫹3v2共16⫹16v⫹3v2兲兴

⫺ 2兩A1兩v

共兩A1兩2⫹v2兲4关兩A1兩

4

v4共288⫹304v⫺25v2兲

⫹兩A1兩6v2192176v17v2

⫹8兩A1兩8共6⫹4vv2兲⫹3v8共16⫹16v⫹3v2兲

⫹兩A1兩2v6192208v41v2兲兴

⫺关16兩A1兩2共2⫹4vv2兲⫹6v2共16⫹16v⫹3v2兲兴

⫻arctan

v

A1兩

. 共D3兲

The more compact form 关Eq. 共38兲兴 is the result of the re-placementv2/s, followed by a number of partial integra-tions.

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Figure

FIG. 1. Sketch of a waveguide containing a randomly scatteringmedium and illuminated by a monochromatic plane wave
FIG. 2. Distribution of the single-mode delay time �diffusive regime. The result of numerical simulationwith�tween the casecirclesmodes14��� in the �data points� N�50 propagating modes is compared to the prediction �Eq
FIG. 3. Distribution of the single-mode delay time �localized regime. The results of numerical simulations with� in the N
FIG. 4. Distribution of the single-mode delay time �forandnegative values oflocalized regime for preserved time-reversal symmetry, in the limitNfrom the solid curve forrescaled by a factor 1.35→ n� in the�
+3

References

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