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Ames Laboratory Accepted Manuscripts Ames Laboratory

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Figure

FIG. 1. (a) The comparison between CaFe2order (the upper panel for real space), and derived two FS pocketsin the vicinity of theSolid and dotted lines denote differences in the orbital occupationwhich induce a static quadrupole moment on the Fe sites with
FIG. 2. Raman spectra for single-crystal CaKFe47 K. TheAs4 at 40 and XY and XX polarized spectra are offset by 1 and 2 units,respectively
TABLE I. Summary of fitting result at 7 K, units in meV.
FIG. 4. Temperature evolution of phonon spectra. (a) The B(c) Temperature dependence of2Aphonon spectra and the fitting curve for above (40 K) and below(7 K)in (a)

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