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(1)

Magnetic dynamics driven by spin current

Group of NonLinear

Magnetic Dynamics

Sergej O. Demokritov

University of Muenster, Germany

(2)

Charge current vs spin current

Electron: possesses both electric charge and spin (angular momentum)

Electronics is based on the flow of charge of electrons.

For an electric circuit we need

sources of electric current

(battery), conductors for

electron flow (metallic wire),

detectors of the current (lamp)

Battery

(3)

Charge current vs spin current

Electron: possesses both electric charge and spin

Spintronics is based on the flow of spin of electrons.

Do we have sources of spin current (battery), conductors for spin flow,

detectors of the spin current (spin-lamp)?

(4)

Spin-polarized vs pure spin current

Electron: possesses both electric charge and spin.

Since spin is a vector, we can separate electric and spin currents.

Electric current: motion of electrons with disordered spins

Spin-polarized current: motion of electrons with

ordered spins.

Pure spin current: motion of ordered spin without

motion of charge.

(5)

Spin-polarized electric current

Spin-up and spin-down

electrons equally

contribute to the current

Non-polarized electric current

I

H H

Symmetry with respect to

spin-up and spin-down is broken

(6)

Spin-polarized electric current

(7)

Spin-polarized electric current

Does spin-polarized electric current have advantages? YES!!!

Giant Magnetoresistance (GMR) effect.

If electrons are injected in a

ferromagnet they can freely move

or will be strongly scattered

depending on the orientation

of their spins with respect to the

magnetization

(8)

Spin-polarized electric current

Does spin-polarized electric current have advantages? YES!!!

Giant Magnetoresistance (GMR) effect.

If electrons are injected in a

ferromagnet they can freely move

or will be strongly scattered

depending on the orientation

of their spins with respect to the

magnetization

R

r

R

r

r

r

R

R

2

2

2

2

2

2

2

2

AP P

R

r

R

R

R

r

r

R

rR

R

r

R

r

r

R

r

R





(9)

Spin-polarized electric current

Does spin-polarized electric current have advantages? YES!!!

Albert Fert

Peter Grünberg

The Nobel Prize in Physics 2007 was awarded jointly to Albert Fert and Peter Grünberg "for the discovery of Giant Magnetoresistance"

Giant Magnetoresistance (GMR) effect.

(10)

Spin current between FM and non-magnetic metal

No spin current at the equilibrium

M

T

T

Spin current due to magnetization

dynamics (spin-pumping)

M

T

T

Spin current due to temperature

gradient (spin Seebeck effect)

M

T

1

T

2

Spin current caused by charge

current (spin Hall effect)

M

T

T

j

S

j

S

j

S

j

c

NM

FM

NM

FM

NM

FM

NM

FM

(11)

Spin current between FM and non-magnetic metal

No spin current at the equilibrium

M

T

T

Spin current due to magnetization

dynamics (spin-pumping)

M

T

T

Spin current due to temperature

gradient (spin Seebeck effect)

M

T

1

T

2

Spin current caused by charge

current (spin Hall effect)

M

T

T

j

S

j

S

j

S

j

c

NM

FM

NM

FM

NM

FM

NM

FM

(12)

Spin-battery: Spin Hall effect

Ordinary Hall effect: separation of particles with

positive and negative charges.

Spin Hall effect: separation of particles with

spin up and down.

due to

SL

 

(13)

Spin Hall vs inverse spin Hall

Spin Hall Effect

spin current battery

c

j

s

j

SHE

c

j

ISHE

Spin Hall Effect

spin current detector

(14)

Magnetic dynamics of ferromagnets

It is described by the Landau-Lifshitz-Gilbert equation

0

 

dm

dm

m

H

m

dt

dt

where 

0

is the Gilbert damping constant (spin-lattice relaxation)

Damping is due to transfer of the angular momentum from

magnetic system to the lattice.

If one applies a dynamic magnetic field with a correct frequency, a

persistent precession can be achieved.

Relaxation of magnetic moment to the lattice is compensated by

the torque of the dynamic field

S

M

H

Static: magnetization is aligned along the magnetic field

m

dm

dt

( )

M t

S

M

H

The dynamic of a ferromagnet: precession

of the magnetization around the field.

(15)

Ferromagnetic resonance (FMR)

By sweeping the magnetic field

(frequency of the precession) one

can recoird the FMR-line.

H

(16)

Ferromagnetic resonance (FMR)

By sweeping the magnetic field

(frequency of the precession) one

can recoird the FMR-line.

H

(17)

Test devices

Disk: Permalloy (Py), 2 m, 5 nm thick Microstrip: Pt, 2.5 m wide, 10 nm thick

dc current is applied through the Pt strip.

The operation of the device relies on the

spin Hall effect (SHE) induced by electrical current in the Pt strip.

SHE produces a spin current at the interface with the Py dot, exerting spin transfer torque (STT) on its magnetization.

Depending on the direction of the current, spin current either

stabilizes or destabilizes the magnetization.

SHE originates from

spin-orbit scattering

resulting in a deflection of conduction electrons with opposite spin

orientations in opposite directions. Permalloy (Py) disk dc current dc current [ + microwave current ]

(18)

Measurement technique

To detect the magnetization dynamics we use

micro-focus Brillouin Light Scattering (BLS) spectroscopy.

1. Probing laser light is focused onto the surface of the magnetic film into a diffraction-limited spot.

2. Light scattered from magnetic excitations is analyzed.

BLS signal is proportional to the

square of the dynamic magnetization

at the position of the probing light spot.

Probing laser light dc current [ + microwave current ] Permalloy (Py) disk

Available resolutions: 1. Frequency resolution 0.05-1000 GHz 2. Temporal resolution < 400 ps

3. Spatial resolution < 250/50 nm 4. Wavevector resolution < 106 cm-1

(19)

Brillouin light scattering process

= inelastic scattering of photons from spin

waves

Conservation laws:

 Time invariance  sc = L

 In-plane translational invariance  qSCqLq

scattered photon phonon or spin wave incident photon wL± w qL± q ® ® w, q® wL, qL ® Spinwellenfrequenz Frequenzverschiebung [GHz] anti-Stokes Stokes B L S -Z ä h lr a te [ C o u n ts ]

(20)

Brillouin spectrometer

-w w magnetic field sample polarization analyser FP1

argon ion laser polarization

rotator

FP2

scanning stage tandem Fabry-Perot interferometer

scan direction spatial filters objective lens acousto-optic modulator prism avalanche photodiode with shutter PC control - stabilisation - data accumulation and processing - display

(21)

Control of effective damping in FMR

Frequency, GHz 7.0 7.5 8.0 8.5 9.0 9.5 10.0 BL S I n te n s ity , a .u .

The FMR curve recorded without the dc current shows a linewidth of

360 MHz at H=900 Oe.

This corresponds to Gilbert damping parameter =0.011, which is close to the

standard value =0.008 for Permalloy.

Microwave current + dc Probing light dc=0 FWHM 360 MHz =0.011 I=-25 mA I=20 mA Frequency, GHz 7.0 7.5 8.0 8.5 9.0 9.5 10.0 BL S In te n s it y , a .u . 0.00 0.25 0.50 0.75 1.00 I=0 mA I=-20 mA I=10 mA

Positive current: broadening of the FMR peak and reduction of its amplitude.

Effect of the current

Negative current: increase of the amplitude and narrowing of the peak.

(22)

FMR Linewidth I, mA -30 -20 -10 0 10 20 30 Li new id th , G H z 0.0 0.2 0.4 0.6 0.8 Continuous Pulsed

The linewidth practically does not depend on whether the current is constant or pulsed (influence of the heating is negligible).  Dependence of the linewidth on I can be attributed entirely to the effect of the spin current.

I, mA -30 -20 -10 0 10 20 30  0.000 0.005 0.010 0.015 0.020 0.025 Continuous Pulsed

Effective Gilbert damping parameter

The achieved variation of  is more than by a factor of 4. The smallest achieved =0.004 is by a factor of 2 smaller

than the standard value for Permalloy.

2 ( 2 e) f H M      

Linewidth shows strong variation with current.  The effect of the spin current on the damping is not significantly reduced by the presence of the Cu spacer.

(23)

To compensate completely

the dynamic

damping

and to achieve excitation of coherent magnetization

dynamics by spin current

without

application of

microwaves

(24)

Control of magnetic fluctuations

dc current

+ microwave current

Thermally-excited unifrom fluctuations are detected by BLS.

BLS spectra exhibit a peak

with a Lorentzian shape. I=-25 mA

I=0 (x2) I=25 mA

(x2)

The amplitude of the peak decreases at I>0 and

increases at I<0.

The linewidth varies linearly with current at small I.

These behaviors are typical for modification of the effective damping by STT. I, mA -30 -20 -10 0 10 20 30 f, GH z 0.5 1.0 1.5

(25)

Control of magnetic fluctuations

Phys. Rev. Lett. 107, 107204 (2011).

The integral under the measured peak is proportional to the average fluctuation energy in the mode.

At I=-28 mA, the integral intensity increases by more than a factor of 30, and at I=28 mA it decreases by more than a factor of 2.

Besides modifying the damping, STT changes the energy of magnetic fluctuations.

This phenomenon can be used for effective “cooling” of a magnetic system and provides practical ways for reduction of thermal noise in magnetic nano-devices.

In agreement with the non-equilibrium theory, the inverse integral intensity shows linear dependence on the current. At I=Ic=-28 mA the integral intensity is expected to diverge

(onset of auto-oscillations).

Instead, it saturates and starts to decrease at I<-26 mA.

Close to the auto-oscillation onset, the flow of energy into the uniform mode saturates, whereas short-wavelength modes

are further enhanced.

Time-resolved measurements

(26)

Auto-oscillations due to spin current

Nature Mater. 11, 1028 (2012).

H

dc current I

Probing spot is positioned in the gap.

Spectral BLS intensity is measured for different I.

Spectrum of thermal magnetic fluctuations.

Low-frequency

modes are enhanced stronger (frequency-dependent radiation losses).

With increasing I the fluctuations are enhanced.

The intensity of

fluctuations diverges as the current approaches a critical value Ic16.1 mA (no saturation).

At I=Ic, a new peak appears in the BLS spectrum.

H=900 Oe

(27)

Spin-Hall nano-oscillator

Nature Mater. 11, 1028 (2012). After the onset of auto-oscillations

Increase of I by 1.3% results in dramatic increase of the intensity of the new peak –

onset of auto-oscillations

The peak rapidly grows and then saturates above 16.3 mA.

Onset of auto-oscillations is accompanied by a decrease in the intensity of thermal fluctuations.

Electronic measurements with similar devices, PRL 110 147601 (2013):

Oscillation Linewidth is 5 MHz at 7 GHz (T=50 K) – proof of high coherence degree

FWHM 5 MHz

(28)

Self-localization of the oscillations

Auto-oscillation mode

To characterize the auto-oscillation mode, we

performed two-dimensional mapping of the dynamic magnetization at the frequency of auto-oscillations.

We rastered the probing laser spot in the two lateral

directions and simultaneously recorded the BLS intensity.

Nature Mater. 11, 1028 (2012).

Auto-oscillations are localized in a very small area in the gap between the electrodes.

H

dc current I

H=900 Oe

The measured spatial distribution is a result of convolution

with the instrumental function determined by the shape of the

laser spot (250 nm).

The real size of the auto-oscillation area is less than 100 nm, significantly smaller than the characteristic size of the current localization.

The auto-oscillation mode is the nonlinear self-localized spin-wave “bullet”.

(29)

Switching using spin current

Using spin current one can switch the magnetization

(30)

Acknowledgement

European Comission

Vladislav E. Demidov, Oleksandr Dzyapko

University of Muenster, Germany

Sergei Urazhdin

Department of Physics, Emery University, Atlanta, USA

M. D. Stiles, R. D. McMichael

NIST, Gaithersburg, USA

V. Tiberkevich, A. Slavin

References

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