• No results found

In this appendix we derive explicit expressions for the scattered two-photon density matrix in Eq. (6.9), recapitulated,

ρ(out)qr,q′r′ = X

klk′l

AklA∗

k′l′uqkurlu∗q′k′u∗r′l′. (6.13)

The random unitary matrix ensemble will be used for averaging over different real- izations of disorder. Any unitary integral of the form

ua1b1...uanbnu∗c1d1...u

cndn

is nonzero if and only ifc∈P(a) andd∈P(b), whereP(x) is the collection of all different permutations ofx, [147, 148]. Logically, there are four essentially different

nonzero second-order integrals possible, being [147, 148] α1 ≡ u11u11u∗11u∗11= 2M M2(M+ 1), (6.14) α2 ≡ u11u12u∗11u∗12= M M2(M+ 1), (6.15) α3 ≡ u11u22u∗11u∗22= M2 M2(M+ 1)(M 1), (6.16) α4 ≡ u11u22u∗12u∗21= − M M2(M+ 1)(M 1), (6.17)

where M is the dimension of the random unitary matrix. When applying this knowledge to Eq. (6.13) it is found that the density matrix elements can take four different values ρ(out)qr,q′r′ =                    X klk′l′ AklA∗ k′l′uqkuqlu∗qk′uql∗′ , q=q′ =r=r′ X klk′l′ AklA∗ k′l′uqkurlu∗qk′u∗rl′ ,(q=q′)6= (r=r′) X klk′l′ AklA∗ k′l′uqkurlu∗rk′u∗ql′ ,(q=r′)6= (r=q′) 0 ,elsewhere. (6.18)

Now it is a matter of bookkeeping to perform the summation and using the integrals in Eqs. (6.14)-(6.17). The nonzero contributions in the summations of Eq. (6.18) are listed in Tab. 6.2. By applying this list to Eq. (6.18) we obtain

ρ(out)qr,q′r′ =            α1D+α2(T − D) +α2(S − D) , q=q′=r=r′ α2D+α3(T − D) +α4(S − D) ,(q=q′)6= (r=r′) α2D+α4(T − D) +α3(S − D) ,(q=r′)6= (r=q′) 0 ,elsewhere , (6.19)

where we introduced three functionals of the inputAkl being

T ≡ M X k=1 M X l=1 AklA∗ kl (6.20) D ≡ M X k=1 AkkA∗ kk, (6.21) S ≡ M X k=1 M X l=1 AklA∗lk. (6.22)

uqkuqlu∗

qk′u∗ql′ uqkurlu∗qk′u∗rl′ uqkurlu∗rk′u∗ql

k=l=k′=lα1 α2 α2

(k=k′)6= (l=l) α2 α3 α4

(k=l′)6= (l=k) α2 α4 α3

Table 6.2: Listing of nonzero outcomes for the three unitary integrals in Eq. (6.18) for different combinations of the summation indicesk,l,k′, andl(note thatq6=r). The coefficientsα

i are defined in Eqs. (6.14)-(6.17).

The symbolsT, D ∈[0,T], and S ∈[−(T − D),+(T − D)] stand fortotal power, diagonal power, andsymmetry parameter, respectively.

By substituting Eqs. (6.14)-(6.17) for the unitary integralsαi in Eq. (6.19) we find ρ(out)qr,q′r′ =                    1 M T +S M+ 1 , q=q′=r=r′ 1 M(M−1) M T − S M+ 1 ,(q=q′)6= (r=r) 1 M(M−1) M S − T M+ 1 ,(q=r′)6= (r=q) 0 ,elsewhere (6.23)

We now make two remarks of mathematical interest. The first remark is thatT and S are functionals ofAkl that are conserved under transformation via any unitary scattering matrix. This can easily be demonstrated by combining the appropriate elements ofρ(out)qr,qr to obtain the averageT andS in the output state being

T(out) = X qr ρ(out)qr,qr=M ρ (out) 11,11+M(M −1)ρ (out) 12,12=T, (6.24) S(out) = X qr ρ(out)qr,rq=M ρ (out) 11,11+M(M −1)ρ (out) 12,21=S. (6.25)

The second remark is that the unitary integrals in Eqs. (6.14)-(6.17) are uniquely determined by stating thatT is a conserved quantity for anyM and any Akl. In other words, by combining Eqs. (6.24) and (6.19) one retrieves Eqs. (6.14)-(6.17). Actually, the unitary integrals are also uniquely determined by stating thatS is a conserved quantity for anyM and anyAkl. So by combining Eqs. (6.25) and (6.19) one retrieves Eqs. (6.14)-(6.17) as well.

Finally, we restrict ourselves to T = 1, which corresponds to normalized two- photon quantum states in Eq. (6.1). Furthermore, we concentrate on the on- diagonal elements of the scattered density matrix only. The relative strength of

these elements is given by the ratio F ≡ ρ (out) 11,11 ρ(out)12,12 = 1 +S 1 + 1− S M−1 , (6.26)

which we will call the pairing factor, whereS ∈[−1,1] andF ∈[0,2]. The pairing factor is the two-photon detection probability observed with two detectors looking into the same spatial channel divided by the two-photon detection probability ob- served with two detectors looking into different spatial channels. Explicit values for these probabilities are easily retrieved by using

Trρ(out)qr,q′r′ =M ρ (out)

11,11+M(M−1)ρ (out)

12,12= 1, (6.27)

[1] J. C. Maxwell, A dynamical theory of the electromagnetic field, Phil. Trans. Roy. Soc. Lond.155, 459 (1865).

[2] J. D. Jackson,Classical electrodynamics, 3 ed. (John Wiley & Sons, Hoboken, NJ, 1999).

[3] L. Mandel and E. Wolf, Optical Coherence and Quantum Optics(Cambridge University Press, The Pitt Building, Trumpington Street, Cambridge, 1995). [4] R. Loudon,The quantum theory of light, 3 ed. (Oxford University Press, Great

Clarendon Street, Oxford, 2000).

[5] R. J. Glauber,The quantum theory of optical coherence, Phys. Rev.130, 2529 (1963).

[6] D. C. Burnham and D. L. Weinberg, Observation of Simultaneity in Para- metric Production of Optical Photon Pairs, Phys. Rev. Lett.25, 84 (1970). [7] R. Ghosh and L. Mandel,Observation of Nonclassical Effects of in the Inter-

ference of Two Photons, Phys. Rev. Lett.59, 1903 (1987).

[8] C. K. Hong, Z. Y. Ou, and L. Mandel,Measurement of subpicosecond time in- tervals between two photons by interference, Phys. Rev. Lett.59, 2044 (1987). [9] C. K. Law and J. H. Eberly, Analysis and Interpretation of High Transverse Entanglement in Optical Parametric Down Conversion, Phys. Rev. Lett.92, 127903 (2004).

[10] H. Di Lorenzo Pires, C. H. Monken, and M. P. van Exter, Direct measure- ment of transverse-mode entanglement in two-photon states, Phys. Rev. A80, 022307 (2009).

[11] H. Bechmann-Pasquinucci and W. Tittel,Quantum cryptography using larger alphabets, Phys. Rev. A61, 062308 (2000).

[12] D. Kaszlikowski, P. Gnaci´nski, M. ˙Zukowski, W. Miklaszewski, and A. Zeilinger,Violations of Local Realism by Two EntangledN-Dimensional Sys- tems Are Stronger than for Two Qubits, Phys. Rev. Lett.85, 4418 (2000). [13] D. Collins, N. Gisin, N. Linden, S. Massar, and S. Popescu, Bell Inequalities

for Arbitrarily High-Dimensional Systems, Phys. Rev. Lett.88, 040404 (2002). [14] L. Zhang, C. Silberhorn, and I. A. Walmsley, Secure Quantum Key Distri- bution using Continuous Variables of Single Photons, Phys. Rev. Lett. 100, 110504 (2008).

[15] L. Allen, M. W. Beijersbergen, R. J. C. Spreeuw, and J. P. Woerdman,Orbital angular momentum of light and the transformation of Laguerre-Gaussian laser modes, Phys. Rev. A45, 8185 (1992).

[16] A. Mair, A. Vaziri, G. Weihs, and A. Zeilinger,Entanglement of the orbital angular momentum states of photons, Nature412, 313 (2001).

[17] G. Molina-Terriza, J. P. Torres, and L.Torner,Orbital angular momentum of photons in noncollinear parametric downconversion, Opt. Comm. 228, 155 (2003).

[18] S. S. R. Oemrawsingh, X. Ma, D. Voigt, A. Aiello, E. R. Eliel, G. W. ’t Hooft, and J. P. Woerdman,Experimental Demonstration of Fractional Orbital An- gular Momentum Entanglement of Two Photons, Phys. Rev. Lett.95, 240501 (2005).

[19] G. Molina-Terriza, J. P. Torres, and L.Torner,Twisted Photons, Nature Phys. 3, 305 (2007).

[20] M. V. Vasnetsov, J. P. Torres, D. V. Petrov, and L. Torner,Observation of the orbital angular momentum spectrum of a light beam, Opt. Lett. 28, 2285 (2003).

[21] R. Zambrini and S. M. Barnett,Quasi-Intrinsic Angular Momentum and the Measurement of Its Spectrum, Phys. Rev. Lett.96, 113901 (2006).

[22] M. P. van Exter, P. S. K. Lee, S. Doesburg, and J. P. Woerdman, Mode Counting in High Dimensional Orbital Angular Momentum Entanglement, Opt. Express15, 6431 (2007).

[23] P. H. Souto Ribeiro, C. H. Monken, and G. A. Barbosa, Measurement of coherence area in parametric downconversion luminescence, Appl. Opt. 33, 352 (1994).

[24] C. K. Hong and T. G. Noh,Two-photon double-slit interference experiment, J. Opt. Soc. Am. B15, 1192 (1998).

[25] T. G. Noh and C. K. Hong, Manifestation of complementarity in double-slit interference, J. Korean Phys. Soc.33, 383 (1998).

[26] E. J. S. Fonseca, C. H. Monken, and S. P´adua,Measurement of the de Broglie wavelength of a multiphoton wavepacket, Phys. Rev. Lett.82, 2868 (1999). [27] E. J. S. Fonseca, C. H. Monken, S. P´adua, and G. A. Barbosa, Transverse

coherence length of down-converted light in the two-photon state, Phys. Rev. A59, 1608 (1999).

[28] E. J. S. Fonseca, J. C. Machado da Silva, C. H. Monken, and S. P´adua, Controlling two-particle conditional interference, Phys. Rev. A 61, 023801 (2000).

[29] A. F. Abouraddy, M. B. Nasr, B. E. A. Saleh, A. V. Sergienko, and M. C. Teich, Demonstration of the complementarity of one- and two-photon inter- ference, Phys. Rev. A63, 063803 (2001).

[30] M. D’Angelo, M. V. Chekhova, and Y. Shih,Two-photon diffraction and quan- tum lithography, Phys. Rev. Lett.87, 013602 (2001).

[31] W. A. T. Nogueira, S. P. Walborn, S. P´adua, and C. H. Monken,Experimental Observation of Spatial Antibunching of Photons, Phys. Rev. Lett. 86, 4009 (2001).

[32] G. Lima, F. A. Torres-Ruiz, L. Neves, A. Delgado, C. Saavedra, and S. P´adua, State determination for composite systems of two spatial qubits, J. Phys.: Con- ference Series84, 012012 (2007).

[33] L. Neves, G. Lima, E. J. S. Fonseca, L. Davidovich, and S. P´adua, Charac- terizing entanglement in qubits created with spatially correlated twin photons, Phys. Rev. A76, 032314 (2007).

[34] R. Shimizu, T. Yamaguchi, Y. Mitsumori, H. Kosaka, and K. Edamatsu, Generation of polarization entanglement from spatially correlated photons in spontaneous parametric down-conversion, Phys. Rev. A77, 032338 (2008). [35] G. Taguchi, T. Dougakiuchi, N. Yoshimoto, K. Kasai, M. Iinuma, H. F. Hof-

mann, and Y. Kadoya,Measurement and control of spatial qubits generated by passing photons through double slits, Phys. Rev. A78, 012307 (2008). [36] C. W. J. Beenakker, J. W. F. Venderbos, and M. P. van Exter, Two-Photon

Speckle as a Probe of Multi-Dimensional Entanglement, Phys. Rev. Lett.102, 193601 (2009).

[37] Y. Lahini, Y. Bromberg, D. N. Christodoulides, and Y. Silberberg,Quantum Correlations in Two-Particle Anderson Localization, Phys. Rev. Lett. 105, 163905 (2010).

[38] J. R. Ott, N. A. Mortensen, and P. Lodahl,Quantum Interference and Entan- glement Induced by Multiple Scattering of Light, Phys. Rev. Lett.105, 090501 (2010).

[39] M. C. W. van Rossum and T. M. Nieuwenhuizen,Multiple scattering of clas- sical waves: microscopy, mesoscopy, and diffusion, Rev. Mod. Phys.71, 313 (1999).

[40] E. Akkermans and G. Montambaux,Mesoscopic physics of electrons and pho- tons(Cambridge University Press, The Edinburgh Building, Cambridge CB2 8RU, UK, 2007).

[41] J. W. Goodman, Speckle Phenomena in Optics: Theory and Applications (Roberts and Company Publishers, Greenwood Village, CO, 2007).

[42] M. P. van Albada and A. Lagendijk, Observation of Weak Localization of Light in a Random Medium, Phys. Rev. Lett.55, 2692 (1985).

[43] C. M. Aegerter and G. Maret, Coherent Backscattering and Anderson Local- ization of Light, Progr. in Opt.52, 1 (2009).

[44] F. Scheffold and G. Maret, Universal Conductance Fluctuations of Light, Phys. Rev. Lett.81, 5800 (1998).

[45] P. W. Anderson, Absence of diffusion in certain random lattices, Phys. Rev. 109, 1492 (1958).

[46] M. St¨orzer, P. Gross, C. M. Aegerter, and G. Maret,Observation of the Criti- cal Regime Near Anderson Localization of Light, Phys. Rev. Lett.96, 063904 (2006).

[47] A. Lagendijk, B. van Tiggelen, and D. S. Wiersema,Fifty years of Anderson localization, Physics Today62, 24 (2009).

[48] A. V. Belinskii and D. N. Klyshko,Two-photon optics: diffraction, hologra- phy, and transformation of two-dimensional signals, Sov. Phys. JETP78, 259 (1994).

[49] J. H. Shapiro and K. X. Sun,Semiclassical versus quantum behavior in fourth- order interference, J. Opt. Soc. B 11, 1130 (1994).

[50] B. I. Erkmen and J. H. Shapiro, Unified theory of ghost imaging with Gaussian-state light, Phys. Rev. A77, 043809 (2008).

[51] C. K. Hong and L. Mandel,Theory of parametric frequency down-conversion of light, Phys. Rev. A31, 2409 (1985).

[52] D. N. Klyshko, Effect of focusing on photon correlation in parametric light scattering, Sov. Phys. JETP 67, 1131 (1988).

[53] Z. Y. Ou, L. J. Wang, and L. Mandel, Vacuum effects on interference in two-photon down conversion, Phys. Rev. A 40, 1428 (1989).

[54] M. H. Rubin, D. N. Klyshko, Y. H. Shih, and A. V. Sergienko, Theory of two-photon entanglement in type-II optical parametric down-conversion, Phys. Rev. A50, 5122 (1994).

[55] A. V. Belinskii and D. N. Klyshko,Two-Photon Wave Packets, Laser Phys. 4, 663 (1994).

[56] M. H. Rubin,Transverse correlation in optical spontaneous parametric down- conversion, Phys. Rev. A54, 5349 (1996).

[57] V. Giovannetti, L. Maccone, J. H. Shapiro, and F. N. C. Wong, Generating Entangled Two-Photon States with Coincident Frequencies, Phys. Rev. Lett. 88, 183602 (2002).

[58] J. H. Shapiro,Quantum Gaussian Noise, Proc. SPIE5111, 382 (2003). [59] Y. Shih, Entangled biphoton source - property and preparation, Rep. Prog.

Phys.66, 1009 (2003).

[60] A. Gatti, R. Zambrini, M. San Miguel, and L. A. Lugiato,Multiphoton mul- timode polarization entanglement in parametric down-conversion, Phys. Rev. A68, 053807 (2003).

[61] D. Z. Cao, Z. Li, Y. H. Zhai, and K. Wang, One-photon and two-photon double-slit interference in spontaneous and stimulated parametric down con- version, Eur. Phys. J. D33, 137 (2005).

[62] F. N. C. Wong, J. H. Shapiro, and T. Kim, Efficient Generation of Polarization-Entangled Photons in a Nonlinear Crystal, Laser Phys.16, 1517 (2006).

[63] Z. Y. Jeff Ou, Multi-Photon Quantum Interference (Springer, 233 Springer Street, New York, 2007).

[64] A. Gatti, E. Brambilla, L. Caspani, O. Jedrkiewicz, and L. A. Lugiato, X

Entanglement: The Nonfactorable Spatiotemporal Structure of Biphoton Cor- relation, Phys. Rev. Lett.102, 223601 (2009).

[65] S. P. Walborn, C. H. Monken, S. P´adua, and P. H. Souto Ribeiro, Spa- tial correlations in parametric down-conversion, Phys. Rep. [Article in press doi:10.1016/j.physrep.2010.06.003] (2010).

[66] B. I. Erkmen and J. H. Shapiro,Gaussian state theory of two-photon imaging, Phys. Rev. A78, 023835 (2008).

[67] E. Brambilla, A. Gatti, M. Bache, and L. A. Lugiato,Simultaneous near-field and far-field spatial quantum correlations in the high-gain regime of paramet- ric down-conversion, Phys. Rev. A69, 023802 (2004).

[68] T. B. Pittman, D. V. Strekalov, D. N. Klyshko, M. H. Rubin, A. V. Sergienko, and Y. H. Shih,Two-photon geometric optics, Phys. Rev. A53, 2804 (1996). [69] C. H. Monken, P. H. S. Ribeiro, and S. P´adua,Transfer of angular spectrum and image formation in spontaneous parametric down-conversion, Phys. Rev. A57, 3123 (1998).

[70] A. E. Siegman,Lasers(University Science Books, Sausalito, 1986).

[71] D. N. Klyshko,Combined EPR and two-slit experiments: interference of ad- vanced waves, Phys. Lett. A132, 299 (1988).

[72] P. G. Kwiat, K. Mattle, H. Weinfurter, A. Zeilinger, A. V. Sergienko, and Y. Shih,New High-intensity source of polarization entangled photon pairs, Phys. Rev. Lett.75, 4337 (1995).

[73] N. Gisin, G. Ribordy, W. Tittel, and H. Zbinden, Quantum cryptography, Rev. Mod. Phys.74, 145 (2002).

[74] S. P. Walborn, A. N. de Oliveira, S. P´adua, and C. H. Monken, Multimode Hong-Ou-Mandel Interference, Phys. Rev. Lett.90, 143601 (2003).

[75] D. P. Caetano and P. H. Souto Ribeiro, Generation of spatial antibunching with free-propagating twin beams, Phys. Rev. A68, 043806 (2003).

[76] W. A. T. Nogueira, S. P. Walborn, S. P´adua, and C. H. Monken,Generation of a Two-Photon Singlet Beam, Phys. Rev. Lett.92, 043602 (2004).

[77] N. K. Langford, R. B. Dalton, M. D. Harvey, J. L. O’Brien, G. J. Pryde, A. Gilchrist, S. D. Bartlett, and A. G. White, , Phys. Rev. Lett.93, 053601 (2004).

[78] B. E. A. Saleh, A. F. Abouraddy, A. V. Sergienko, and M. C. Teich,Duality between partial coherence and partial entanglement, Phys. Rev. A62, 043816 (2000).

[79] P. S. K. Lee and M. P. van Exter, Spatial labeling in a two-photon interfer- ometer, Phys. Rev. A73, 063827 (2006).

[80] M. P. van Exter, A. Aiello, S. S. R. Oemrawsingh, G. Nienhuis, and J. P. Woerdman, Effect of spatial filtering on Schmidt decomposition of entangled photons, Phys. Rev. A74, 012309 (2006).

[81] J. P. Torres, A. Alexandrescu, and L. Torner, Quantum spiral bandwidth of entangled two-photon states, Phys. Rev. A68, 050301 (2003).

[82] R. Grobe, K. Rzazewski, and J. H. Eberly,Measure of electron-electron cor- relation in atomic physics, J. Phys. B27, L503 (1994).

[83] A. Ekert and P. L. Knight,Entangled quantum-systems and the Schmidt de- composition, Am. J. Phys.63, 415 (1995).

[84] S. Franke-Arnold, S. M. Barnett, M. J. Padgett, and L. Allen, Two-photon entanglement of orbital angular momentum states, Phys. Rev. A 65, 033823 (2002).

[85] L. Torner, J. P. Torres, and S. Carrasco,Digital spiral imaging, Opt. Express 13, 873 (2005).

[86] M. Segev, R. Solomon, and A. Yariv,Manifestation of Berry’s phase in image- bearing optical beams, Phys. Rev. Lett.69, 590 (1992).

[87] M. W. Beijersbergen, R. P. C. Coerwinkel, M. Kristensen, and J. P. Woerd- man, Helical-wavefront laser beams produced with a spiral phaseplate, Opt. Comm.112, 321 (1994).

[88] S. S. R. Oemrawsingh, J. A. W. van Houwelingen, E. R. Eliel, J. P. Woerdman, E. J. K. Verstegen, J. G. Kloosterboer, and G. W. ’t Hooft,Production and characterization of spiral phase plates for optical wavelengths, Appl. Opt.43, 688 (2004).

[89] M. M. Fejer, G. A. Magel, D. H. Jundt, and R. L. Byer,Quasi-phase-matched second harmonic generation: tuning and tolerances, IEEE J. Quantum Elec- tron.28, 2631 (1992).

[90] M. Hou´e and P. D. Townsend,An introduction to methods of periodic poling for second-harmonic generation, J. Phys. D: Appl. Phys.28, 1747 (1995). [91] C. Canalias, V. Pasiskevicius, and F. Laurell,Periodic Poling of KTiOPO4:

From Micrometer to Sub-Micrometer Domain Gratings, Ferroelectrics340, 27 (2006).

[92] F. Laurell, M. G. Roelofs, W. Bindloss, H. Hsiung, A. Suna, and J. D. Bierlein, Detection of ferroelectric domain reversal in KTiOPO4 waveguides, J. Appl.

Phys.71, 15 (1992).

[93] H. Bluhm, A. Wadas, R. Wiesendanger, A. Roshko, J. A. Aust, and D. Nam, Imaging of domain-inverted gratings in LiNbO3 by electrostatic force microscopy., Appl. Phys. Lett. 71, 146 (1997).

[94] G. Rosenman, A. Skliar, I. Lareah, N. Angert, M. Tseitlin, and M. Roth,Ob- servation of ferroelectric domain structures by secondary-electron microscopy in as-grown KTiOPO4, Phys. Rev. B 54, 6222 (1996).

[95] C. Canalias, V. Pasiskevicius, A. Fragemann, and F. Laurell,High-resolution domain imaging on the nonpolar y-face of periodically poled KTiOPO4 by means of atomic force microscopy., Appl. Phys. Lett.83, 734 (2003).

[96] S. K. Johansen and P. Baldi,Characterization of quasi-phase-matching grat- ings in quadratic media through double-pass second-harmonic power measure- ments, J. Opt. Soc. Am. B21, 1137 (2004).

[97] I. Cristiani, C. Liberale, V. Degiorgio, G. Tartarini, and P. Bassi, Nonlinear characterization and modeling of periodically poled lithium niobate waveguides for 1.5-µm-band cascaded wavelength conversion, Opt. Commun. 187, 263 (2001).

[98] S. J. Holmgren, V. Pasiskevicius, S. Wang, and F. Laurell,Three-dimensional characterization of the effective second-order nonlinearity in periodically poled crystals, Opt. Lett.28, 1555 (2003).

[99] G. K. H. Kitaeva, V. V. Tishkova, I. I. Naumova, A. N. Penin, C. H. Kang, and S. H. Tang,Mapping of periodically poled crystals via spontaneous parametric down conversion, Appl. Phys. B81, 645 (2005).

[100] P. D. Maker, R. W. Terhune, M. Nisenoff, and C. M. Savage,Effects of disper- sion and focussing on the production of optical harmonics, Phys. Rev. Lett. 8, 21 (1962).

[101] S. Emanueli and A. Arie, Temperature-dependent dispersion equations for KTiOPO4 and KTiOAsO4, Appl. Opt.42, 6661 (2003).

[102] F. Pignatiello, M. D. Rosa, P. Ferraro, S. Grilli, P. D. Natale, A. Arie, and S. D. Nicola,Measurement of the thermal expansion coefficients of ferroelectric crystals by a moir´e interferometer, Opt. Commun.227, 14 (2007).

[103] T. Y. Fan, C. E. Huang, B. Q. Hu, R. C. Eckardt, Y. X. Fan, R. L. Byer, and R. S. Feigelson,Second harmonic generation and accurate index of refraction